3.5 - Precise interferometry of glass plates

Study on the factors affecting the refractive index change of chalcogenide films induced by femtosecond laser

Due to the limitations of measurement equipment and the influence of factors such as the environment and target, measurement errors may occur during the data acquisition process of airborne LiDAR bathymetry (ALB). The refractive index of water is defined as the propagation ratio of the speed of light waves in a vacuum to that in water; this ratio influences not only the propagation speed of the laser pulse in water but also the propagation direction of the laser pulse entering water. Therefore, the influence of refractive index changes in water on the ALB errors needs to be analyzed. To this end, the principle of ALB is first briefly introduced. Then, the calculation method for the refractive index of water is described with Snell’s law and an empirical formula. Finally, the influence of refractive index changes on ALB errors is analyzed using the derived formula at the water–air interface and in the water column. The experimental results showed that in a constant elevation of 50 m for a bathymetric floor, the refractive index changes in water caused by temperature, salinity, and depth are less than 0.001. The maximum bathymetric error and maximum planimetric error caused by the refractive index changes at the water–air interface are 0.036 m and 0.015 m, respectively. The ALB errors caused by refractive index changes in the water column are relatively low, and the water column does not need to be layered to calculate the ALB errors. The influence of refractive index changes in water on the ALB error is minimal, accounting for only a small proportion of all bathymetric errors. Thus, it is necessary to determine whether the effect of the ALB error due to refractive index changes in water needs to be corrected based on the accuracy requirements of the data acquisition. This study and analysis can provide a reference basis for correcting ALB errors.

The refractive index changes induced by stimulated Brillouin scattering in an optical fiber are measured experimentally by polarization-decoupled four-wave mixing. Under undepleted pump approximation, net phase-matching condition depends on pump power and frequency detuning from Brillouin frequency. By investigating this net phase-matching condition, one can measure spectral change in the refractive index which is responsible for the slow light effect based on stimulated Brillouin scattering. Due to the high sensitivity of the measurement, very small refractive index changes (on the order of 10^-8) versus frequency detuning can be determined experimentally, which is the lowest index change reported so far.

Here, we demonstrate the preparation of a hybrid nanoplasmonic probe array, a nanoforest, which consists of gold nanostructures coated on top of silica nanospheres and evaporated gold film structure onto bottom through masks. Optically tunable plasmonic surfaces could be achieved by varying the nanoforest fabrication conditions, which acted as a selective nanoantenna. Plasmon coupling effects were effectively controlled by adjusting the vertical distance (nanogap) between the gold nanostructures on the silica bead and the bottom. Such control is critical to highly sensitive molecular detection applications. As a proof of concept, nanoforests were used as colorimetric sensors of refractive index changes. The sensors were highly sensitive and displayed distinct colors for small refractive index (RI) changes. The flexible and sensitive near/far-field optical properties render these nanoforests excellent plasmonic substrates for quantitative, sensitive and label-free sensing with nanoscale spatial resolution.

We analyze the transmission property of nanostructures made on silver and gold metal for the applications in optical biosensors. Various structures such as slit only, slit groove slit, and multiple slit and groove structures are taken into account to find the effect of various physical parameters such as number of grooves, number of slits and others on the transmission of different wavelength light sources through the structure. A broad wavelength of 400 nm to 900 nm is used to analyze the transmission through the structure. With these structures and broad light source, change in transmission intensity is analyzed with the change in the refractive index. The change in refractive index of the analyte varies transmission intensity and wavelength shift at the output beam which can be used for sensing the amount of analyte such as monitoring glucose amount on blood/saliva, hydrogen peroxide and others. The detection of these analytes can be used to detect the different disease. The analysis of the transmittance through the nanostructure can be used for the detection of several disease such as diabetes and others through the saliva, blood and others non-invasively.

Common-path spectral-domain optical low coherence interferometric system for the measurement of small changes in refractive index of Liquid Crystal cell

An optical waveguide sensor was fabricated by forming a multilayer film made by porous anodic alumina (PAA) and Al layers on a glass substrate. The fabricated sensor system was based on the monitoring of a waveguide coupling mode, which is sensitive to the change in the refractive index of the PAA layer caused by collection of target molecules into the pores of the PAA layer. The PAA/Al multilayer film was formed by partial anodization of an Al film deposited on the glass substrate, and the waveguide coupling mode was examined by measuring angular spectra (reflectivity dependence on the incident angle of monitoring light; green He-Ne laser, 534.5 nm). A deep and sharp waveguide coupling dip was obtained for the PAA/Al multilayer system where the thicknesses of the PAA and Al layers were 200 and 17 nm, respectively. The optical sensor response of the PAA/Al multilayer system was compared to the responses of a surface plasmon resonance (SPR) sensor made by a Au thin film on a SF10 glass substrate. It was inferred that the optical waveguide sensor made by the PAA/Al multilayer could detect a smaller change in the refractive index of a solution, and it provided higher resolution than the SPR sensor. The sensor response for a change in the complex refractive index of the PAA layer was examined next, and it was found that the optical waveguide sensor was sensitive to the change in the imaginary part of the complex refractive index rather than the change in the real part. This result indicated that the sensitivity of the optical waveguide sensor could be improved by using the light absorption of a target compound.

This study explores how hydrostatic pressure, temperature, incident light intensity, and structural parameters modulate optical absorption coefficients and refractive index changes in GaAs/Al0.3Ga0.7As spherical quantum dots under the screened cosine Kratzer potential. We use the Nikiforov-Uvarov method to solve the Schrödinger equation to determine the relevant wave functions and energy levels. And using iterative method and density matrix theory, we derived analytical expressions for the optical absorption coefficients and refractive index changes. The results of the numerical analyses demonstrate that both the structural parameters of the quantum dots and the external environmental factors significantly influence the optical absorption coefficients and refractive index changes, with varying degrees of impact. It is particularly noteworthy that these factors are extremely important for modulating the peak amplitude and resonance peak position of the optical absorption coefficients and refractive index changes, providing important theoretical basis for us to deeply understand and modulate the nonlinear optical properties of quantum dots.

Intersubband optical absorption coefficients and refractive index changes in modulation-doped asymmetric double quantum well

The surface plasmon resonance (SPR) signal, generated from the Kretschmann configuration, has been developed as an effective detection technology in chemical and biological sensors. The sensitivity of SPR signals to changes in the surrounding media makes it a valuable tool, as even a slight variation in refractive index can cause a significant change in SPR signals, such as phase, intensity, and resonance angle. However, the detection of ultralow changes in refractive index, which occur in chemical reactions or biological actions, remains a challenge for conventional SPR sensors due to their limited sensitivity. To overcome this limitation, we theoretically propose a novel guided-wave SPR (GWSPR) configuration coated with a few-layer blue phosphorene (blueP)/MoS2 hybrid structure. This configuration aims to enhance the electric field and subsequently achieve a significant improvement in sensitivity. The results of our study demonstrate that the proposed blueP/MoS2-based GWSPR sensor exhibits a high sensitivity of 290°/RIU, which represents an impressive enhancement of approximately 82.4% compared to the conventional Au-based SPR sensor. This advancement addresses the challenge of detecting ultralow changes in refractive index and offers significant potential for enhancing the performance of chemical and biological sensors.

A new concept for the detection of very small changes in the refractive index of a small sample of transparent material is given. The concept is based on measuring the frequency difference between two modes of a laser (possibly a twin- laser), where the evanescent field of one mode is affected by small refractive index changes. Intracavity sensing allows for orders of magnitude greater sensitivity than with external sensing. The frequency difference is obtained by light beating of the two modes. An imbedded diffractive element ensures proper modematching for the light beating. The relative frequency change is equal to the relative change in refractive index properly averaged over the waveguide. The performance of the intracavity system is compared with a system based on a Mach-Zehnder interferometer. The intracavity system may achieve a resolution that is 104 - 106 higher than the sensitivity of a system based on an external interferometer. The effect of thermal instability is investigated and it is discussed how the required very low thermal off-set can be maintained. Injection locking can be a problem. The problem may be solved by either introducing a fixed frequency off- set or by proper design of the cavity structure. An implementation based on III-V materials with a waveguide configuration and Bragg-mirrors is possible with existing technologies. A concept based on a polymer configuration is proposed.© (1998) COPYRIGHT SPIE--The International Society for Optical Engineering. Downloading of the abstract is permitted for personal use only.

Integrated optical Mach-Zehnder interferometers supply information on changes in refractive index and/or thickness of a film placed as a superstrate on top of one of its surface wave-guides. The internal propagation of light is influenced by the evanescent field reaching into the superstrate. This propagating light interferes with an uninfluenced wave in the second arm after recombination. The result is an intensity modulation depending on the refractive index parameters of the substrate, the waveguide itself and the properties of the superstrate. Taking an antigen layer as the superstrate, its interaction with antibodies changes its thickness by several nanometers. This can be observed by recording the change in intensity of the signal of the interferometer. The sensitivity of such a device depends on particular values of the optical parameters of substrate and waveguide with respect to the given superstrate properties. Computer calculations help to select optimum glass and waveguide fabrication conditions. The numerical results of a variety of assumed conditions have been tested experimentally. The application to the improved detection of triazines is discussed.

Understanding and controlling laser-induced refractive index modifications in bulk chalcogenide glasses is important for a range of photonics applications targeting the mid-infrared spectral region. We focus here on material engineering aspects and pulse spatio-temporal design characteristics that are able to induce and maintain positive refractive index changes in laser-irradiated Sulfur-based chalcogenide glass, mandatory for 3D photonic design. Specifically we study the photoinscription process of a Ge-doped Sulfur-based chalcogenide glass, Ge15As15S70, irradiated by focused ultrafast near-infrared laser pulses where Ge doping plays a determinant role in generating high-contrast positive index changes. By means of aposteriori and real-time in situ observations we show that positive refractive index changes (type I) are the result of a restructuring of the glass matrix and a photo-induced contraction process initiated by two-photon electronic excitation leading to bond softening, molecular mobility, structural changes and rearrangements. Oppositely, negative refractive index changes (type II) could be associated with two different processes: photo-expansion at higher intensities and hydrodynamic evolution initiated by plasma generation and laser heating, with thermomechanical relaxation and stress unload. Alongside the role of Ge in setting various degrees of the matrix connectivity, the structural arrangement developed under different thermal history schemes for glass preparation is equally important as it defines to which extent further structural flexibility is possible. Thus we indicate the role of glass matrix metastability in generated high-contrast refractive index changes and we show that a higher degree of relaxation is an impediment for contrasted positive index changes, while these are developing in unrelaxed glasses, where several degrees of structural flexibility exist. Alongside dynamic time-resolved imaging experiments probing the development and relaxation of excitation, we also show, via static Raman analysis of the modified regions, that significant structural changes are induced by laser irradiation and we discuss the potential processes involved.

Cytoplasmic viscosity is a crucial parameter in determining rates of diffusion-limited reactions. Changes in viscosity are associated with several diseases, whilst nuclear viscosity determines gene integrity, regulation and expression. Yet how drugs including DNA-damaging agents affect viscosity is unknown. We demonstrate the use of a platinum complex, Pt[L]Cl, that localizes efficiently mostly in the nucleus as a probe for nuclear viscosity. The phosphorescence lifetime of Pt[L]Cl is sensitive to viscosity and provides an excellent tool to investigate the impact of DNA damage. We show using Fluorescence Lifetime Imaging (FLIM) that the lifetime of both green and red fluorescent proteins (FP) are also sensitive to changes in cellular viscosity and refractive index. However, Pt[L]Cl proved to be a more sensitive viscosity probe, by virtue of microsecond phosphorescence lifetime versus nanosecond fluorescence lifetime of FP, hence greater sensitivity to bimolecular reactions. DNA damage was inflicted by either a two-photon excitation, one-photon excitation microbeam and X-rays. DNA damage of live cells causes significant increase in the lifetime of either Pt[L]Cl (HeLa cells, 12.5–14.1 µs) or intracellularly expressed mCherry (HEK293 cells, 1.54–1.67 ns), but a decrease in fluorescence lifetime of GFP from 2.65 to 2.29 ns (in V15B cells). These values represent a viscosity change from 8.59 to 20.56 cP as well as significant changes in the refractive index (RI), according to independent calibration. Interestingly DNA damage localized to a submicron region following a laser microbeam induction showed a whole cell viscosity change, with those in the nucleus being greater than the cytoplasm. We also found evidence of a by-stander effect, whereby adjacent un-irradiated cells also showed nuclear viscosity change. Finally, an increase in viscosity following DNA damage was also observed in bacterial cells with an over-expressed mNeonGreen FP, evidenced by the change in its lifetime from 2.8 to 2.4 ns.

Self phase modulation is a nonlinear effect that is observed when a laser beam is focused on to a high-absorbing thermal medium. A regular tea sample in a plastic cuvette is used as the nonlinear absorbing sample. The change in the refractive index of the medium occurs due to the heat generated by the focused pump beam, which in turn changes the refractive index. In this paper, self phase modulation is investigated in different ways. An Ar-Ion laser of 514 nm is used as the pump beam and a 632 nm He-Ne laser is used as the probe beam. The probe beam is introduced from the opposite side of the pump beam. Ring patterns are observed from the each side of the sample. Regular far field ring patterns are observed from the pump beam, and two sets of rings are observed with the probe beam. The behaviors of these inner and outer rings are monitored for different pump powers. The steady state heat equation is solved to obtain an exact solution for the radial heat distribution and far field ring patterns are simulated using the Fresnel–Kirchhoff diffraction integral. Ring patterns are theoretically explained using simulations results, and compared with experimental observations. Finally, an interferometric setup using the low power He-Ne laser is also used to determine the induced change in refractive index. Results are compared with those obtained directly from self-phase modulation and from the probe beam method.