An Introduction to All-Optical Quantum Controlled-NOT Gates

In NMR quantum computing, spin states of spin-1/2 nuclei are called qubits. Quantum logic gates are represented by unitary matrices. As a universal gate, controlled-NOT (CNOT) is a two-qubit gate. For the IS (I = 1/2 and S = 1/2) spin system, two-qubit CNOT gate is represented by a 4 × 4 matrix. SWAP logic gate, which exchanges two quantum states, is constructed by CNOT gates. In this study, first, four-qubit CNOT gates are constructed for the IS (I = 3/2, S = 3/2) spin system. Then, by using these CNOT gates, a four-qubit SWAP logic gate is found. As an application and verification, an obtained SWAP logic gate is applied to the matrix representation of product operators for the IS (I = 3/2, S = 3/2) spin system. SWAP logic gate can also be presented by an NMR pulse sequence. By using the product operator theory, the pulse sequence of the SWAP logic gate is applied to product operators of the IS (I = 3/2, S = 3/2) spin system. The expected exchange results are obtained for both the matrix representation and the pulse sequence of SWAP logic gate.

The Controlled-NOT (CNOT) quantum gate associated with single qubit gates is universal for building all quantum circuits. Although CNOTs based on trapped ions and superconducting qubits have become experimentally feasible, the deterministically functioning quantum CNOT gate with photonic qubits will lead to practical realization of quantum computers in a deterministic manner, and will therefore provide an exponential increase in processing power with lowest decoherence time. Based on a previously proposed CNOT model utilizing a quantum cloner (with a fidelity of 78 %), we present in this work our design of the Compact CNOT gate providing a fidelity of 90.31 %, and give physical realization constraints for building CNOT based decomposition of the Toffoli gate and more generalized photonic CnNOT gates. The photonic qubits are encoded by circularly polarized single photons and the design of the gate is based on copying the polarization degree of freedom by quantum cloners. Our model is based on spin of electron in a quantum dot embedded in a double sided optical microcavity which behaves like a beam splitter. Circularly polarizing beam splitters, beam splitters, delay lines, photonic circulators, single qubit operations and other photonic devices are used for the design and decomposition. We show that the fidelity of the decomposed CnNOT gates is highly dependent on the errors of the non-perfect photonic devices used and more specifically to the theoretical optimal limit of 5/6 of the quantum cloners required for each CNOT in the decomposition.

Linear optics quantum computing (LOQC) is a leading candidate for the implementation of large scale quantum computers. Here quantum information is encoded into the quantum states of light and computation proceeds via a linear optics network. It is well known that in such schemes there are stringent requirements on the spatio-temporal structure of photons -- they must be completely indistinguishable and of very high purity. We show that in the Boson-sampling model for LOQC these conditions may be significantly relaxed. We present evidence that by increasing the size of the system we can implement a computationally hard algorithm even if our photons have arbitrarily low fidelity and purity. These relaxed conditions make Boson-sampling LOQC within reach of present-day technology.

Unlike classical digital computers in which a bit can represent either 1 or 0 at any time, quantum computers use a two-level system, i.e., a qubit, to implement logical operations based on quantum mechanical laws, which can represent both values at once. Owing to the superposition property of qubits, quantum computers have natural parallel processing advantages and thus have potential to exceed the computational efficiency of classical computers for particular tasks. Quantum logic gates are the generalization of classical logic gates in computational networks. It has been proved that two-qubit quantum gates together with one-qubit quantum gates are adequate for constructing networks with any possible quantum computational property. Directional couplers are the most critical elementsfor constructing the quantum gates. In recent years, photonic quantum technologies have emerged as a promising experimental platform for quantum computing. Single photons have robust noise resistance, long coherence time, high transmission speed and great compatibility with other systems. They can be easily manipulated and encoded in any of several degrees of freedom, for example, polarization, path, spatial mode or time bin. Optical waveguide technology enables the realizing of complex optical schemes comprised of many elements with desired scalability, stability and miniaturization. Femtosecond laser direct writing of waveguide has been adopted as a powerful tool for integrated quantum photonics with characteristics of rapidness, cost-effectiveness, mask-less and single-step process. In particular, it has the ability to build arbitrary three-dimensional circuits directly inside bulk materials, which is impossible to achieve with conventional lithography. In this article we review the femtosecond laser writing and quantum characterization of directional coupler and important one-qubit and two-qubit optical quantum logic gates, such as Hadamard gate, Pauli-X gate, controlled-NOT gate, and controlled-Phase gate. The qubits in these gates are usually encoded through optical paths or polarizations of photons. The key to the realization of polarization-encoded one-qubit gates is to achieve flexible wave-plate operations, which is described in detail. Controlled-NOT gate and controlled-phase gate are the most crucial two-qubit gates in the linear optics computation and sometimes they can be converted into each other by adding some one-qubit gates or special superposition states. Many different kinds of waveguide circuits have been used to implement these two-qubit gates. The outlook and challenges for the femtosecond laser writing of three-qubit gates, such as Toffoli gate and Fredkin gate, are briefly introduced.

A basic experiment on 2-bit quantum calculations related to the Deutsch–Jozsa algorithm on a linear optical quantum computer using a liquid crystal (LC) device as a linear optical element was investigated. By controlling the phase of each of the two split laser beams and checking the number of photons at the output, it is possible to determine if the input bits are “not equal” or “not uniform.” The phase of the laser light was controlled using an LC device and a half-wave plate, and changes in the interference state of the output light and the number of photons were observed. The voltage application to the LC device is set at the input bit. As a result, the interference state changed according to the input bit, and changes in the number of photons were observed.

We present a scheme for linear optical quantum computation that is highly robust to imperfect single photon sources and inefficient detectors. In particular we show that if the product of the detector efficiency with the source efficiency is greater than 2/3, then efficient linear optical quantum computation is possible. This high threshold is achieved within the cluster state paradigm for quantum computation.

We propose a scheme for efficient cluster state quantum computation by using imperfect polarization-entangled photon-pair sources, linear optical elements and inefficient non-photon-number-resolving detectors. The efficiency threshold for loss tolerance in our scheme requires the product of source and detector efficiencies should be >1/2 - the best known figure. This figure applies to uncorrelated loss. We further find that the loss threshold is unaffected by correlated loss in the photon pair source. Our approach sheds new light on efficient linear optical quantum computation with imperfect experimental conditions.

Entangled photons are a crucial resource for linear optical quantum communication and quantum computation. Besides the remarkable progress of photon state engineering using atomic memories (Kimble (2008); Yuan et al. (2008)) the majority of current experiments is based on the production of photon pairs in the process of spontaneous parametric down-conversion (SPDC), where the entangled photon pair is concluded from post-selection of randomly occurring coincidences. Here we present new insights into the heralded generation of photon states (Barz et al. (2010); Wagenknecht et al. (2010)) that are maximally entangled in polarization (Schrodinger (1935)) with linear optics and standard photon detection from SPDC (Kwiat et al. (1995)). We utilize the down-conversion state corresponding to the generation of three pairs of photons, where the coincident detection of four auxiliary photons unambiguously heralds the successful preparation of the entangled state (Śliwa & Banaszek (2003)). This controlled generation of entangled photon states is a significant step towards the applicability of a linear optics quantum network (Nielsen & Chuang (2000)), in particular for entanglement distribution (Bennett et al. (1996)), entanglement swapping (Kaltenbaek et al. (2009); Pan et al. (1998)), quantum teleportation (Bouwmeester et al. (1997)), quantum cryptography (Bennett & Brassard (1984); Ekert (1991); Jennewein et al. (2000)) and scalable approaches towards photonics-based quantum computing schemes (Browne & Rudolph (2004); Gottesman & Chuang (1999); Knill et al. (2001)).

Quantum information has been witnessing great science value and latent application since 1980's. The research work presented here consist of mainly two important parts: manipulations of multiphoton entanglement and atomic ensembles based quantum memory. In first part, the experimental technique multi-photon entanglement is further developed to study fundamental issues in quantum mechanics, remarkable applications to quantum communication and quantum computation. Specifically, we have demonstrated a bit-flip error-free transfer of quantum information, violation of Bell's inequality beyond Tsirelson's bound, teleportation of a two-qubit composite system, as well as the one-way computing by two-photon-four-qubit cluster state. To overcome un-scalability problem due to probabilistic feature in linear optical quantum information processing, we investigated in the second part the physics of atomic ensembles based quantum memory. We show that theoretically, entanglement between distant locations can be deterministically generated. The experimental work has thoroughly developed the necessary techniques and we have achieved deterministic single photon source, and interference of the photons from independent atomic ensembles, teleportation between photonic and atomic qubits, a novel way to create a robust entanglement between an atomic and a photonic qubit, and memory based entanglement swapping. We believe, the developed techniques here would dramatically facilitate progresses in many fields including global quantum communication, linear optical quantum computation and the foundations of quantum mechanics etc.

Quantum emitters are an integral component for a broad range of quantum technologies, including quantum communication, quantum repeaters, and linear optical quantum computation. Solid-state color centers are promising candidates for scalable quantum optics due to their long coherence time and small inhomogeneous broadening. However, once excited, color centers often decay through phonon-assisted processes, limiting the efficiency of single-photon generation and photon-mediated entanglement generation. Herein, we demonstrate strong enhancement of spontaneous emission rate of a single silicon-vacancy center in diamond embedded within a monolithic optical cavity, reaching a regime in which the excited-state lifetime is dominated by spontaneous emission into the cavity mode. We observe 10-fold lifetime reduction and 42-fold enhancement in emission intensity when the cavity is tuned into resonance with the optical transition of a single silicon-vacancy center, corresponding to 90% of the excited-state energy decay occurring through spontaneous emission into the cavity mode. We also demonstrate the largest coupling strength (g/2π = 4.9 ± 0.3 GHz) and cooperativity (C = 1.4) to date for color-center-based cavity quantum electrodynamics systems, bringing the system closer to the strong coupling regime.

The creation of specified quantum states is important for most, if not all, applications in quantum computation and communication. The quality of the state preparation is therefore an essential ingredient in any assessment of a quantum-state gun. We show that the fidelity, under the standard definitions is not sufficient to assess quantum sources, and we propose a new measure of suitability that necessarily depends on the application for the source. We consider the performance of single-photon guns in the context of quantum key distribution (QKD) and linear optical quantum computation. Single-photon sources for QKD need radically different properties than sources for quantum computing. Furthermore, the suitability for single-photon guns is discussed explicitly in terms of experimentally accessible criteria.

We show that with the addition of multiple walkers, quantum walks on a line can be transformed into lattice graphs of higher dimension. Thus, multi-walker walks can simulate single-walker walks on higher dimensional graphs and vice versa. This exponential complexity opens up new applications for present-day quantum walk experiments. We discuss the applications of such higher-dimensional structures and how they relate to linear optics quantum computing. In particular we show that multi-walker quantum walks are equivalent to the BosonSampling model for linear optics quantum computation proposed by Aaronson & Arkhipov. With the addition of control over phase-defects in the lattice, which can be simulated with entangling gates, asymmetric lattice structures can be constructed which are universal for quantum computation.

We demonstrate how gradient ascent pulse engineering optimal control methods can be implemented on donor electron spin qubits in Si semiconductors with an architecture complementary to the original Kane's proposal. We focus on the high-fidelity controlled-NOT (CNOT) gate and explicitly find its digitized control sequences by optimizing its fidelity over the external controls of the hyperfine A and exchange J interactions. This high-fidelity CNOT gate has an error of about $10^{-6}$, below the error threshold required for fault-tolerant quantum computation, and its operation time of 100ns is about 3 times faster than 297ns of the proposed global control scheme. It also relaxes significantly the stringent distance constraint of two neighboring donor atoms of 10~20nm as reported in the original Kane's proposal to about 30nm in which surface A and J gates may be built with current fabrication technology. The effects of the control voltage fluctuations, the dipole-dipole interaction and the electron spin decoherence on the CNOT gate fidelity are also discussed.

We present a feasible and efficient scheme, and its proof-of-principle demonstration, of creating entangled photon pairs in an event-ready way using only simple linear optical elements and single photons. The quality of entangled photon pair produced in our experiment is confirmed by a strict violation of Bell's inequality. This scheme and the associated experimental techniques present an important step toward linear optics quantum computation.

Quantum information technology has been developing rapidly in last two decades. Very recently, quite a few optical quantum key distribution networks have been reported, enabling preliminary practical applications in secure information transfer. Meanwhile, a number of significant progresses based on quantum network have also been made in the research of linear optical quantum computing, simulation and metrology. However, on the way towards large-scale optical quantum network serious problems occur. On the one hand, the distance of fiber-based quantum communication is limited, due to intrinsic fiber loss and decreasing of entanglement quality caused by the noisy environment. On the other hand, the probabilistic feature of single and entangled photon sources would also cause an exponentially increasing overhead for large-scale quantum network. To solve the above problems, quantum repeaters and/or transmission of optical quantum bits over free space channel can be efficiently exploited for future wide-area realization of quantum communication. In addition, memory built-in quantum repeaters would also enable scalable linear optical quantum computing, simulation and high precision measurement. In this talk I will present some recent experiments from our group, including eight-photon entanglement, topological quantum error-correction, quantum repeater and efficient and long-lived quantum memory, and entanglement distribution and quantum teleportation over 100km-scale free-space quantum channels. These experiments show the promising future possibility towards scalable quantum network with photons and atoms.