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  • https://doi.org/10.1021/acsphotonics.5c01526Copy DOI Icon

Influence ofDriving Pulse Properties on Third-HarmonicDiffraction from Quasi-BIC Metasurfaces

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Abstract

Quasi-bound states in the continuum in dielectric metasurfacessupport sharp Fano resonances that emerge from the interference betweenbrightand dark modes. We exploit this modal interplay to demonstrate tunablethird-harmonic emission, controlled through the driving pulse’swavelength and intensity. Our experiments show imbalances in third-harmonicdiffraction patterns and non-Gaussian third-harmonic spectral featuresthat exhibit strong variations near the Fano resonance. We explainthe observations via a coupled-oscillator model that captures theinterplay between the driving field and the nonlinear response ofthe modes, explaining our observations and providing a predictiveframework for optimizing the third-harmonic diffraction efficiency.These results establish pulse-engineered metasurfaces as a powerfulplatform for nonlinear wavefront shaping and frequency conversionapplications while simultaneously serving as a warning that pulseproperties play a vital role in metasurface function design.

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