Multi-photon entanglement: from quantum curiosity to quantum computing and quantum repeaters

Quantum information has been witnessing great science value and latent application since 1980's. The research work presented here consist of mainly two important parts: manipulations of multiphoton entanglement and atomic ensembles based quantum memory. In first part, the experimental technique multi-photon entanglement is further developed to study fundamental issues in quantum mechanics, remarkable applications to quantum communication and quantum computation. Specifically, we have demonstrated a bit-flip error-free transfer of quantum information, violation of Bell's inequality beyond Tsirelson's bound, teleportation of a two-qubit composite system, as well as the one-way computing by two-photon-four-qubit cluster state. To overcome un-scalability problem due to probabilistic feature in linear optical quantum information processing, we investigated in the second part the physics of atomic ensembles based quantum memory. We show that theoretically, entanglement between distant locations can be deterministically generated. The experimental work has thoroughly developed the necessary techniques and we have achieved deterministic single photon source, and interference of the photons from independent atomic ensembles, teleportation between photonic and atomic qubits, a novel way to create a robust entanglement between an atomic and a photonic qubit, and memory based entanglement swapping. We believe, the developed techniques here would dramatically facilitate progresses in many fields including global quantum communication, linear optical quantum computation and the foundations of quantum mechanics etc.

Entangled photon sources play a pivotal role in most of the optical systems that utilize quantum effects. Those include quantum key distribution, quantum computing, metrology, sensing and imaging. Photon pair generation using spontaneous parametric down conversion (SPDC) is one of the most popular routes for producing entangled photons. While SPDC has become more popular, the creation of entangled photon pairs in a degree of freedom, such as polarization, is more challenging. The difficulty is related in no small part to the birefringence of the structure where the generation takes place. Birefringence results in distinguishing information that hinders the production of entanglement in the platforms where SPDC has been most popular including ferroelectric crystals.Despite this limitation, entangled sources have been realized in bulk crystals via well designed interference techniques, which often include additional compensating optics. As the boundaries of optical quantum information science continue to be extended, multi-photon entanglement is now required. Solutions based on SPDC have been attempted, and while some outstanding results have been achieved, the interferometers and compensation procedures become increasingly complex as the size of the entangled state grows. Such scalability and stability issues are directly addressed by integrated entangled photon sources, and while still in their infancy, they promise to help a great deal towards the practical utilization and the production of entanglement on a larger scale.Semiconductors are an ideal platform to fabricate such integrated entangled photon sources. Recently, it was demonstrated that the gallium-arsenide (GaAs) based Bragg refection waveguide (BRW), could efficiently produce photon pairs via SPDC. This platfrom was shown to have a distinct advantage over other semiconductor sources, due largely to its monolithic architecture and its layered epitaxy, which underpins many photonic devices. In this work we demonstrate yet another advantage: the intrinsic capability of the BRW to directly produce polarization entangled photon pairs, without any additional interferometry, spectral filtering, compensation or post-selection. Not only do we show that the BRW can produce entangled photons, but we wish to emphasize that the traditional compensation and interferometric methods used to create entanglement, which presumably would have occurred on chip, may no longer be necessary. Our experimental results confirm that the BRW has the potential to be one of the very first self-contained integrated room temperature resources of entanglement.In this talk various approaches for utilizing SPDC processes in various integration platforms will be discussed. The root cause of entanglement generation is the lack of birefringence in these material systems, which otherwise makes exact phase matching impossible in bulk crystals. Because of this, cross-polarized photons propagate at almost identical group velocities, making off-chip path compensation unnecessary.

Quantum information technology has been developing rapidly in last two decades. Very recently, quite a few optical quantum key distribution networks have been reported, enabling preliminary practical applications in secure information transfer. Meanwhile, a number of significant progresses based on quantum network have also been made in the research of linear optical quantum computing, simulation and metrology. However, on the way towards large-scale optical quantum network serious problems occur. On the one hand, the distance of fiber-based quantum communication is limited, due to intrinsic fiber loss and decreasing of entanglement quality caused by the noisy environment. On the other hand, the probabilistic feature of single and entangled photon sources would also cause an exponentially increasing overhead for large-scale quantum network. To solve the above problems, quantum repeaters and/or transmission of optical quantum bits over free space channel can be efficiently exploited for future wide-area realization of quantum communication. In addition, memory built-in quantum repeaters would also enable scalable linear optical quantum computing, simulation and high precision measurement. In this talk I will present some recent experiments from our group, including eight-photon entanglement, topological quantum error-correction, quantum repeater and efficient and long-lived quantum memory, and entanglement distribution and quantum teleportation over 100km-scale free-space quantum channels. These experiments show the promising future possibility towards scalable quantum network with photons and atoms.

Quantum teleportation is one of the most basic quantum protocols, which transfers an unknown quantum state from one location to another through local operation and classical communication by using shared quantum entanglement without physical transfer of the information carrier. And it has been widely used in various quantum information protocols such as entanglement swapping, quantum repeaters, quantum gate teleportation, quantum computation based on measurement, and quantum teleportation networks, which have important application value in quantum computation and quantum information. Quantum teleportation is a naturally bipartite process, in which an unknown quantum state can only be transmitted from one node to another. With the further development of quantum information research, it is necessary to transfer quantum states or quantum information among more and more nodes. Multipartite quantum protocols are expected to form fundamental components for larger-scale quantum communication and computation. A bipartite quantum teleportation should be extended to a multipartite protocol known as a quantum teleportation network. In this paper, a multifunctional quantum teleportation network is proposed theoretically. We first propose a special method of constructing four-partite quantum resources in continuous variables (CVs), and based on this, construct two different types of CV quantum teleportation networks. One type of network contains just one quantum teleportation process consisting of a sender, a receiver and two controllers. In this type of network, the unknown quantum state can be recovered at any other node according to the requirement after the measurement in the input node, which enriches the transfer direction and transfer mode of the unknown quantum state. And meanwhile, the two controllers can control the transfer of a quantum state from the sender to the receiver by restricting the sender and receiver’s access to their information, which makes the quantum teleportation network controllable. The other type of network has two quantum teleportation processes, each containing only a sender, a receiver and no controllers, which increases the number of quantum states that can be transmitted. Then we analyze the dependence of the fidelity of each quantum teleportation network on different physical parameters, and compare the characteristics, advantages and disadvantages among different types of quantum teleportation networks. The scheme for constructing a multifunctional quantum teleportation network in this paper shows some advantages, such as the greater number of quantum nodes, diversity of types, simple operation procedure. And all these advantages provide a broader application prospect for establishing larger and more complex quantum information networks in the future and quicken the pace of the application of quantum information.

We demonstrate entanglement swapping of polarization entangled photons using an interferometric Bell-state measurement operating at the theoretical limit of 50% efficiency capable of identifying two of the four Bell states. Our experiment represents the highest quality of entanglement swapping so far, with the correlations of the final entangled states showing an overlap fidelity with the ideal Bell states of F = 0.892, and a violation Bell's inequality for both swapped entangled states. In order to achieve this high-quality operation we have optimized various experimental error sources of our setup including the quality of optical elements, as well as the constraints due to the coherence and the group-velocity mismatch of the pump and down-conversion photons. Our results are relevant for experiments that involve interferences of independent photons and pulsed multi-photon states, such as in quantum computing, quantum metrology and quantum communication with quantum repeaters.

Quantum communication relies on the existence of entanglement between two nodes of a network. However, due to its fragile nature, it is nearly impossible to establish entanglement at large distances through the direct transmission of qubits. Quantum repeaters have been proposed to solve this problem, which split-up the network to create small-scale entangled links and then connect them up to create the large-scale link. As researchers race to establish entanglement over larger and larger distances, it becomes essential to gauge the performance and robustness of the different protocols that have been proposed to design a quantum repeater, before deploying them in real life. Currently available noisy quantum computers are ideal for this task, as they can emulate the noisy environment in a quantum communication channel, and provide a measure for how the protocols will perform on real-life hardware. In this paper, we report the circuit-level implementation of the complete architecture of a quantum repeater, and benchmark this protocol on IBM's cloud quantum computer - IBMQ. Our experiments indicate a 26% fidelity of shared bell-pairs for a complete on-chip quantum repeater with a yield of 49%. We also compare these results with simulation data from IBM Qiskit. The results of our experiments provide a quantitative measure for the fidelity of entanglement that currently available repeaters can establish. In addition, the proposed circuit-implementation provides a robust benchmark for state-of-the-art quantum computing hardware.

Quantum information science attempts to exploit capabilities from the quantum realm to accomplish tasks that are otherwise impossible in the classical domain. Although sufficient conditions have been formulated for the physical resources required to achieve quantum computation and communication, there is a growing understanding of the power of quantum measurement combined with the conditional evolution of quantum states for accomplishing diverse tasks in quantum information science. For example, a protocol has recently been developed for the realization of scalable long-distance quantum communication and the distribution of entanglement over quantum networks. Here we report the first enabling step in the realization of this protocol, namely the observation of quantum correlations for photon pairs generated in the collective emission from an atomic ensemble. The nonclassical character of the fields is demonstrated by the violation of an inequality involving their normalized correlation functions. Compared to previous investigations of non-classical correlations for photon pairs produced in atomic cascades and in parametric down-conversion, our experiment is distinct in that the correlated photons are separated by a programmable time interval (of about 400 nanoseconds in our initial experiments).

Quantum computing is a multidisciplinary field at the intersectionof quantum physics, computer science, and mathematics, aiming to har-ness quantum mechanical phenomena for computational advantage. Thisarticle provides a comprehensive review of both the foundational princi-ples and advanced theoretical models of quantum computing. We beginwith the basic framework of quantum computation, introducing the con-cept of qubits as two-level quantum systems, the linear algebra of Hilbertspaces, Dirac’s bra–ket notation, and the postulates of quantum mechan-ics (state superposition, unitary evolution, and projective measurement).We then discuss quantum logic gates and circuits, highlighting how clas-sical reversible computation principles extend to universal quantum gatesets. Next, we survey key quantum algorithms (from Shor’s factoring toGrover’s searching and beyond) and the complexity-theoretic implicationsof quantum computers, contrasting the class BQP with classical complex-ity classes. We cover the theoretical foundations of quantum error cor-rection and fault tolerance, explaining how quantum information can beprotected from decoherence using redundancy and how fault-tolerant pro-tocols can, in principle, allow scalable quantum computation despite noisyhardware. We then explore advanced models and paradigms of quantumcomputation, including measurement-based quantum computing (one-wayquantum computing), topological quantum computation with anyons, adi-abatic quantum computing and quantum annealing, continuous-variablequantum computing, and related approaches. We also provide an overviewof quantum information theory as it relates to computation, discussingentanglement, quantum entropy, and information-theoretic limits like theHolevo bound. Finally, we review the leading physical implementations(quantum hardware models) of quantum computers—trapped ions, super-conducting circuits, photonic systems, solid-state spin qubits, and oth-ers—outlining the challenges and achievements of each approach.

Local Friendliness (LF) inequalities follow from seemingly reasonable assumptions about reality: (i) ``absoluteness of observed events'' (e.g., every observed event happens for all observers) and (ii) ``local agency'' (e.g., free choices can be made uncorrelated with other events outside their future light cone). Extended Wigner's Friend Scenario (EWFS) thought experiments show that textbook quantum mechanics violates these inequalities. Thus, experimental evidence of these violations would make these two assumptions incompatible. In [Nature Physics 16, 1199 (2020)], the authors experimentally implemented an EWFS, using a photonic qubit to play the role of each of the ``friends'' and measured violations of LF. One may question whether a photonic qubit is a physical system that counts as an ``observer'' and thereby question whether the experiment's outcome is significant. Intending to measure increasingly meaningful violations, we propose using a statistical measure called the ``branch factor'' to quantify the ``observerness'' of the system. We then encode the EWFS as a quantum circuit such that the components of the circuit that define the friend are quantum systems of increasing branch factor. We run this circuit on quantum simulators and hardware devices, observing LF violations as the system sizes scale. As errors in quantum computers reduce the significance of the violations, better quantum computers can produce better violations. Our results extend the state of the art in proof-of-concept experimental violations from branch factor 0.0 to branch factor 16.0. This is an initial result in an experimental program for measuring LF violations at increasingly meaningful branch factors using increasingly more powerful quantum processors and networks. We introduce this program as a fundamental science application for near-term and developing quantum technology.

The novel field of quantum computation and quantum information has gathered significant momentum in the last few years. It has the potential to radically impact the future of information technology and influence the development of modern society. The construction of practical, general purpose quantum computers has been challenging, but quantum cryptographic and communication devices have been available in the commercial marketplace for several years. Quantum networks have been built in various cities around the world and a dedicated satellite has been launched by China to provide secure quantum communication. Such new technologies demand rigorous analysis and verification before they can be trusted in safety- and security-critical applications. Experience with classical hardware and software systems has shown the difficulty of achieving robust and reliable implementations. We present CCS q , a concurrent language for describing quantum systems, and develop verification techniques for checking equivalence between CCS q processes. CCS q has well-defined operational and superoperator semantics for protocols that are functional , in the sense of computing a deterministic input-output relation for all interleavings arising from concurrency in the system. We have implemented QEC (Quantum Equivalence Checker), a tool that takes the specification and implementation of quantum protocols, described in CCS q , and automatically checks their equivalence. QEC is the first fully automatic equivalence checking tool for concurrent quantum systems. For efficiency purposes, we restrict ourselves to Clifford operators in the stabilizer formalism, but we are able to verify protocols over all input states. We have specified and verified a collection of interesting and practical quantum protocols, ranging from quantum communication and quantum cryptography to quantum error correction.

Scaling quantum computers, i.e., quantum processing units (QPUs) to enable the execution of large quantum circuits is a major challenge, especially for applications that should provide a quantum advantage over classical algorithms. One approach to scale QPUs is to connect multiple machines through quantum and classical channels to form clusters or even quantum networks. Using this paradigm, several smaller QPUs can collectively execute circuits that each would not be able on its own. However, communication between QPUs is costly as it requires generating and maintaining entanglement, and hence it should be used wisely. In this paper, we evaluate the architectures, and in particular the entanglement patterns, of variational quantum circuits in a distributed quantum computing (DQC) setting. That is, using Qiskit, we simulate the execution of an eight qubit circuit using four QPUs each with two computational and two communication qubits where non-local CX-gates are performed using the remote-CX protocol. We compare the performance of various circuits on a binary classification task where training is executed under ideal and testing under noisy conditions. The study provides initial results on suitable VQC architectures for the DQC paradigm, and indicates that a standard VQC baseline is not always the best choice, and alternative architectures that use entanglement between QPUs sparingly deliver better results under noise.

The complex environment of solid-state quantum bits is generally believed to pose a difficult challenge for solid state realizations of quantum information science. Close study of single electronic spins associated with the nitrogen-vacancy (NV) center in diamond has shown how a complex environment -- in this case a spin-bath formed by carbon-13 isotopic impurities -- may be understood and even controlled. Specifically, we show that optical and microwave excitation of the NV center can be used to perform robust initialization, manipulation, and measurement of the two-qubit register formed by the electronic spin and its nearest-neighbor carbon-13 nuclear spin. These few-qubit registers may be used as a basis for scalable quantum information systems provided that one can identify a means to connect different registers. For an optically active system such as the NV center, photons provide a natural medium for inter- register communication, and we discuss initial experiments studying the possibility of quantum optical interconnects. Such an optically-connected few-qubit register offers a flexible hardware for both quantum computation and long-distance quantum communication; in particular, it may allow realization of a solid-state quantum repeater.

(English) Future networks for quantum communication will require a new form of technology in order to operate over long distances. The no-cloning theorem precludes the use of amplification, so quantum repeater schemes have been proposed to achieve long-distance quantum communication through the distribution of entanglement. A key device for this setup is a quantum memory, which is required in order to store entanglement and synchronise its distribution. Among the many physical systems than can be used as a quantum memory, rare-earth ion-doped crystals stand out due to their long coherence times and potential for multiplexing and integration. This thesis reports the use of one such system, Pr3+:Y2SiO5, as a quantum memory using the atomic frequency comb (AFC) protocol. Building on previous work, we improved the performance of the memory to be able to demonstrate light-matter entanglement with a telecommunications wavelength photon and the quantum memory, for both a bulk memory and an integrated version. To measure light-matter entanglement, we use photon pairs generated through cavity-enhanced spontaneous parametric down conversion, where one photon (the signal) is stored in the memory and the other (the idler) is at a telecommunications wavelength. These photon pairs exhibit energy-time entanglement, which we analyse in the time basis using fibre- and AFC-based Mach-Zehnder interferometers. In the first experiment, we demonstrate light-matter entanglement where the bulk quantum memory is used with on-demand retrieval via storage in a spin-wave. We measure interference fringes with average visibilities of 89(2)% for AFC storage, and 70(3)% for spin-wave storage, sufficient to demonstrate entanglement. This is the first such demonstration using an on-demand multimode solid-state memory and telecom photon. We show that entanglement is maintained for up to 47.7 µs of storage. These results were made possible through improvements in the AFC efficiency and the noise filtering. Furthermore, we perform on-demand storage and retrieval of up to 30 temporal modes. We take the next step towards implementing our system in a real world scenario by measuring entanglement over a distance. To do so, we send the idler photons through both optical fibre spools and deployed fibre in the metropolitan area of Barcelona, Spain, while the photon detection still occurs in the same lab. The resulting visibilities (80% or higher) demonstrate that the photonic qubit does not decohere during transmission through the optical fibre. We then decouple the photon creation and detection by measuring non-classical correlations between signal photons detected in the lab, and idler photons detected 16 km away (44 km in fibre) in a different location. The final experiment uses a fibre-integrated memory for light-matter entanglement. We use a Pr3+:Y2SiO5 crystal containing a Type I laser-written waveguide, interfaced directly with optical fibre. The fibre-integration allows for improved transmission and AFC efficiency compared to a free-space coupled waveguide memory. To analyse the performance of the memory, we demonstrate non-classical correlations for storage times up to 28 µs. We perform qubit tomography in the time basis for storage times of 3 and 10 µs, measuring two-qubit fidelities of 86(2)% and 86(4)%, respectively, demonstrating storage of entanglement. These experiments demonstrate the potential of our system for use as part of a quantum repeater, with many opportunities for further improvement to the storage time, efficiency, and multiplexing capability.

Quantum networks are composed of quantum nodes which coherently interact by way of quantum channels. They offer powerful capabilities for quantum computation, communication, and metrology. A generic requirement for these realizations is the capability to generate and store quantum states among multiple quantum nodes, and to disseminate these resources throughout the network via the quantum channels. In this thesis, I describe a series of experiments whereby single excitations in atomic ensembles are strongly coupled to optical modes and provide efficient means for the coherent control of entangled states between matter and light. By following the seminal proposal by Duan et al., we have generated measurement-induced entanglement of an excitation between two cold atomic ensembles. Using this system, we investigated the relationship for the global bipartite entanglement and local correlations in its subsystems. In addition, we achieved functional quantum nodes for entanglement distribution. Two pairs of remote ensembles at two quantum nodes were prepared into entangled states in a heralded and asynchronous fashion by the conditional controls of the entanglement. The quantum states of the ensembles were then distributed into polarization entangled states of photons. We also prepared an analogous quantum state and transferred the nonlocal coherence between two pairs of heralded entangled atomic ensembles, providing a step towards entanglement connection. Beyond such probabilistic approaches, we demonstrated an experiment where entanglement between two quantum memories is created by the reversible and deterministic mapping of an entangled state of light via dynamic electromagnetically induced transparency. This experiment opens novel prospects of integrating hybrid quantum systems by way of reversible quantum interfaces between light and matter. Then, we extended our work to multipartite quantum systems. We theoretically investigated the characterization of multipartite mode-entangled states by way of quantum uncertainty relations, and introduced theoretical tools to verify the entanglement orders in multipartite systems. In particular, we achieved entanglement for one delocalized photon among multiple optical modes (N > 2). Finally, we have achieved measurement-induced entanglement of spin waves among four quantum memories. The individual atomic components for the entangled W state of the four ensembles were then coherently converted into four propagating entangled beams of light via superradiant emissions. We observed the statistical and dynamic transitions for the multipartite entangled spin waves. Experiments described in this thesis thereby represent significant advances of experimental and theoretical capabilities to generate, store, transfer, and characterize entanglement of matter and light over quantum networks.

Quantum Computer: Quantum Model and Reality