Multimode image memory based on a cold atomic ensemble

Quantum networks are composed of quantum nodes which coherently interact by way of quantum channels. They offer powerful capabilities for quantum computation, communication, and metrology. A generic requirement for these realizations is the capability to generate and store quantum states among multiple quantum nodes, and to disseminate these resources throughout the network via the quantum channels. In this thesis, I describe a series of experiments whereby single excitations in atomic ensembles are strongly coupled to optical modes and provide efficient means for the coherent control of entangled states between matter and light. By following the seminal proposal by Duan et al., we have generated measurement-induced entanglement of an excitation between two cold atomic ensembles. Using this system, we investigated the relationship for the global bipartite entanglement and local correlations in its subsystems. In addition, we achieved functional quantum nodes for entanglement distribution. Two pairs of remote ensembles at two quantum nodes were prepared into entangled states in a heralded and asynchronous fashion by the conditional controls of the entanglement. The quantum states of the ensembles were then distributed into polarization entangled states of photons. We also prepared an analogous quantum state and transferred the nonlocal coherence between two pairs of heralded entangled atomic ensembles, providing a step towards entanglement connection. Beyond such probabilistic approaches, we demonstrated an experiment where entanglement between two quantum memories is created by the reversible and deterministic mapping of an entangled state of light via dynamic electromagnetically induced transparency. This experiment opens novel prospects of integrating hybrid quantum systems by way of reversible quantum interfaces between light and matter. Then, we extended our work to multipartite quantum systems. We theoretically investigated the characterization of multipartite mode-entangled states by way of quantum uncertainty relations, and introduced theoretical tools to verify the entanglement orders in multipartite systems. In particular, we achieved entanglement for one delocalized photon among multiple optical modes (N > 2). Finally, we have achieved measurement-induced entanglement of spin waves among four quantum memories. The individual atomic components for the entangled W state of the four ensembles were then coherently converted into four propagating entangled beams of light via superradiant emissions. We observed the statistical and dynamic transitions for the multipartite entangled spin waves. Experiments described in this thesis thereby represent significant advances of experimental and theoretical capabilities to generate, store, transfer, and characterize entanglement of matter and light over quantum networks.

This thesis is a summary of my research work during the last few years of my Ph.D. The main system of research is quantum memory based on cold atomic ensembles. Flying photons can be used to transmit quantum information over long distances, and quantum memories based on cold atomic ensembles can act as carriers for local storage and manipulation of quantum information, so it is of great significance to study cold atomic quantum memories for construction of global quantum networks. In this thesis, based on previous work, we further scrutinize the factors that will affect the performance metrics of quantum memory such as retrieval efficiency, and then we combine these analysis with some innovative experimental techniques, which will enable us to finally realize a highly retrievable quantum memory with intrinsic retrieval efficiency up to 90% and overall measured retrieval efficiency up to 40%. Based on this efficient quantum memory, we optimize the experimental loading time for preparing cold atomic ensembles, the number of experimental trials in each loading and other timing parameters, so that the experimental detection brightness of photons can support our experimental study of multiple quantum memories.

The reversible transfer of a high-dimensional quantum state between a true single photon, an information carrier, and a matter used as a quantum memory with high fidelity and reliability could enhance the channel capacity significantly in addition to overcoming distance limitations of quantum communication schemes through transmission losses. In the Chap. 2, we have introduced how we demonstrated single photon storage encoded with two-dimensional OAM degree of freedom. Due to the infinity Hilbert space spanned by OAM degree of freedom, photon encoded in OAM space can extend to high-dimensional state. Quantum memories have been realized with different physical systems, such as atomic ensembles and solid systems etc., many of them only realize the storage and retrieval of the single photons spanned in a two-dimensional space for example, orthogonal polarizations, therefore only a quantum bit could be stored there. In this Chapter, I will introduce an experimental realization of a quantum memory storing a heralded photon lived in a three-dimensional space spanned by OAM via EIT in a cold atomic ensemble. We reconstruct the storage process density matrix with fidelity of \(85.3\% \) by the aid of a 4-F imaging system experimentally. The ability to store a high-dimensional quantum state with high fidelity is very promising for building a high-dimensional quantum network.

In the domain of quantum communication, one of the main challenges is the distribution of entanglement over long distances. A scheme, the so-called quantum repeater, has been proposed in order to overcome the problem of channel losses. In this thesis we adresse different problems related to quantum repeaters, both theoretically and experimentally. We present an alternative scheme of quantum repeater based on atomic ensembles and linear optics. It is based on the use of a qubit amplifier and two photon interference. The main features of the protocol are that the distributed entangled state does not need post selection and the entanglement distribution rates approach the optimal rates one might expect from quantum repeaters using probabilistic swapping. An important concern of the whole class of quantum repeaters based on one photon interference is the phase stability in the communication channels. We performed an experiment evaluating the realistic phase noise in installed optical fibers in the Geneva urban area. We found fluctuations of order of 0.1 rad on the time scale of order of 100 $mu$s. The feasibility of the phase stabilization is discussed. One of the essential building blocks of quantum repeater is a quantum memory. We focus our attention on quantum memories based on solid state atomic ensembles and photon echo like techniques. In particular, we show, that the atomic coherence in eryso can be controlled to a very high degree using an external electric field. This allowed us to implement the CRIB protocol in this material and realize the first storage of light at the single photon level at telecommunication wavelength. A necessary step for the implementation of CRIB and AFC storage protocols, in order to achieve long storage times and unit efficiencies, is the use of control light pulses. We developped a numerical Maxwell-Bloch simulator allowing us to study a coherent control of atomic excitations. In particular, we investigate the use of adiabatic chirped pulses in the context of AFC protocol. We study the relationship between the pulse characteristics and the echo properties. The comparison with the conventional $pi$ pulses and the impacts on the multimode capacity of the AFC protocol are also discussed.

In quantum information science, photons are the best candidate for transmitting information, and atoms are the best candidate for storing information. The combination of these two systems provides a fascinating future for practical applications of the quantum information concepts. The work presented in this thesis mainly consists of two parts. The first part is about manipulation of entangled photons, including the demonstration of a nondestructive CNOT gate, the creation of narrowband entangled photons through cavity-enhanced spontaneous parametric down-conversion, and the realization of interference between narrowband photon sources. The second part is about manipulation of atomic ensembles. The main purpose for this part is to extend the quantum communication distance using the concept of quantum repeater. Within this part, the experimental work includes, the extension of storage lifetime of quantum memories to 1 ms by increasing the wavelength of stored spinwave, the realization of entanglement assisted spinwave interferometer, the demonstration of efficient entanglement swapping with quantum memories, and the realization of quantum teleportation between atomic ensembles.

We have demonstrated upconversion detection at the single photon level in the 2 μm spectral window using a pump wavelength near 1550 nm, a periodically poled lithium niobate (PPLN) waveguide, and a volume Bragg grating (VBG) to reduce noise. We achieve a system photon detection efficiency of 10%, with a noise count rate of 24,500 counts per second, competitive with other 2 μm single photon detection technologies. This detector has potential applications in environmental gas monitoring, life science, and classical and quantum communication.

Quantum information technology based on solid state qubits has created much interest in converting quantum states from the microwave to the optical domain. Optical photons, unlike microwave photons, can be transmitted by fiber, making them suitable for long distance quantum communication. Moreover, the optical domain offers access to a large set of very well‐developed quantum optical tools, such as highly efficient single‐photon detectors and long‐lived quantum memories. For a high fidelity microwave to optical transducer, efficient conversion at single photon level and low added noise is needed. Currently, the most promising approaches to build such systems are based on second‐order nonlinear phenomena such as optomechanical and electro‐optic interactions. Alternative approaches, although not yet as efficient, include magneto‐optical coupling and schemes based on isolated quantum systems like atoms, ions, or quantum dots. Herein, the necessary theoretical foundations for the most important microwave‐to‐optical conversion experiments are provided, their implementations are described, and the current limitations and future prospects are discussed.

The parametric interaction of light beams in nonlinear materials is usually thought to be too weak to be observed when the fields involved are at the single-photon level. However, such single-photon level nonlinearity is not only fundamentally fascinating but holds great potential for emerging technologies and applications involving heralding entanglement at a distance. Here we use a high-efficiency waveguide to demonstrate the sum-frequency generation between a single photon and a single-photon level coherent state. The use of an integrated, solid state, room temperature device and telecom wavelengths makes this type of system directly applicable to future quantum communication technologies such as device-independent quantum key distribution.

We discuss recent our recent progress on functional photonic crystals devices and circuits for classical and quantum information processing. For classical applications, we have demonstrated a room-temperature-operated, low threshold, nanocavity laser with pulse width in the picosecond regime; and an all-optical switch controlled with 60 fJ pulses that shows switching time on the order of tens of picoseconds. For quantum information processing, we discuss the promise of quantum networks on multifunctional photonic crystals chips. We also discuss a new coherent probing technique of quantum dots coupled to photonic crystal nanocavities and demonstrate amplitude and phase nonlinearities realized with control beams at the single photon level.

The high-dimensional quantum system greatly improve the quantum channel capacity and information storage space, and achieve high-dimensional quantum information transmission, which enhance the speed of quantum computing and quantum information processing. In this paper, a high-dimensional quantum teleportation protocol without information loss is proposed. We consider pre-sharing a high-dimensional non-maximum entangled state as a quantum channel between sender and receiver. By adding auxiliary particle and performing high-dimensional local operations, it is possible to achieve high-dimensional quantum teleportation without information loss. Simultaneously, we apply the protocol to butterfly network, and propose a novel high-dimensional quantum network coding based on prediction mechanism. In our scheme, we use Z-{|0⟩, |1⟩} basis to predict the transmission of high dimensional states over the butterfly network. When the prediction is successful, the deterministic transmission of high-dimensional quantum states can be realized over the butterfly network. Our scheme greatly saves the usage of quantum and classical channels, which improves the utilization efficiency of both channels.

The full structuration of light in the transverse plane, including intensity, phase and polarization, holds the promise of unprecedented capabilities for applications in classical optics as well as in quantum optics and information sciences. Harnessing special topologies can lead to enhanced focusing, data multiplexing or advanced sensing and metrology. Here we experimentally demonstrate the storage of such spatio-polarization-patterned beams into an optical memory. A set of vectorial vortex modes is generated via liquid crystal cell with topological charge in the optic axis distribution, and preservation of the phase and polarization singularities is demonstrated after retrieval, at the single-photon level. The realized multiple-degree-of-freedom memory can find applications in classical data processing but also in quantum network scenarios where structured states have been shown to provide promising attributes, such as rotational invariance.

The analysis of link loss is one of the first and most important steps for the design of an optical communication system. This is particularly vital in quantum communications systems where the information is encoded at the single photon level, and the quantum optical signal cannot be amplified deterministically. In most cases, the desired quantum bit error rate and secure key rate can only be achieved by minimizing the link attenuation and the background noise level in the quantum communication system. In optical fiber implementations, the transmission distance is inherently limited by the loss per unit distance of the optical fiber, meaning fully global coverage is not readily achievable with the current optical fiber backbone networks. To overcome the terrestrial link limitations for quantum communications, long-distance free-space links, using low-Earth orbit satellites are being proposed and implemented. Due to the optical link length, the main contributors to link losses are geometric loss, atmospheric attenuation, and losses associated with pointing and tracking errors. The total link loss is dominated by the geometric loss, therefore, it is important to analyze its importance in relation to the quantum communications link. In this paper, the loss of a low-Earth orbit satellite-to-ground (downlink) quantum communication link is analyzed. The analysis includes losses associate with the channel (geometric and atmospheric) and the receiver system. This paper also compares the data of a known satellite quantum communications mission, highlighting trade-offs in investment for satellite platform and optical ground station. Based on the link loss analysis, decoy state BB84 and E91 protocols were chosen to demonstrate the link performance under an example scenario. The work contributes to the design of the optical ground station for a CubeSat mission.

Quantum communication provides an absolute security advantage, and it has been widely developed over the past 30years. As an important branch of quantum communication, quantum secure direct communication (QSDC) promotes high security and instantaneousness in communication through directly transmitting messages over a quantum channel. The full implementation of a quantum protocol always requires the ability to control the transfer of a message effectively in the time domain; thus, it is essential to combine QSDC with quantum memory to accomplish the communication task. In this Letter, we report the experimental demonstration of QSDC with state-of-the-art atomic quantum memory for the first time in principle. We use the polarization degrees of freedom of photons as the information carrier, and the fidelity of entanglement decoding is verified as approximately 90%. Our work completes a fundamental step toward practical QSDC and demonstrates a potential application for long-distance quantum communication in a quantum network.

Quantum entanglement is one of the most important resources in quantum information. In recent years, the research of quantum entanglement mainly focused on the increase in the number of entangled qubits or the high-dimensional entanglement of two particles. Compared with qubit states, multipartite high-dimensional entangled states have beneficial properties and are powerful for constructing quantum networks. However, there are few studies on multipartite high-dimensional quantum entanglement due to the difficulty of creating such states. In this paper, we experimentally prepared a multipartite high-dimensional state left|{Psi }_{442}rightrangle =frac{1}{2}(left|000rightrangle +left|110rightrangle +left|221rightrangle +left|331rightrangle ) by using the path mode of photons. We obtain the fidelity F = 0.854 ± 0.007 of the quantum state, which proves a real multipartite high-dimensional entangled state. Finally, we use this quantum state to demonstrate a layered quantum network in principle. Our work highlights another route toward complex quantum networks.

A distributed quantum network requires versatile and high-fidelity quantum memory nodes, but it remains challenging to make them scalable. This study investigates the use of multiple controllable quantum memories in silicon carbide---an established semiconductor material platform for various quantum technology applications---and provides a viable solution. The authors show that solid-state spins in silicon carbide are ideal quantum memories in a distributed quantum computing network, wherein a controlled generation of highly coherent qubit registers using nuclear spins is possible. This study will impact the future development of quantum networks with solid states spins as quantum memories.