Proton acceleration by relativistic self-guided laser pulses

Target normal sheath acceleration (TNSA) by self-guided laser pulses is demonstrated at a range of Al target thickness (2-10 microns), and proton spectra are compared with those accelerated by un-guided laser pulses. For un-guided pulses, the maximum proton energy decreases with the decrease of target thickness, exhibiting the detrimental effect of laser pre-pulse on TNSA. On the other hand, the dependence of proton energy on target thickness was not observed when using self-guided laser pulses, which is possibly due to the suppressed pre-pulse intensity. However the laser pulse appears to lose a significant amount of energy (>~50%) during ~4mm self-guiding in the plasma, and thus the accelerated proton energy is much lower than the case of unguided pulses.

The interaction of short and intense laser pulses with plasmas or solids is a very efficient source of high-energy ions. This paper reports the detailed study, with particle-in-cell simulations, of the interaction of such a laser pulse with thin, dense targets, and the resulting proton acceleration. Depending on the laser intensity and pulse duration, the most energetic protons are found to come from the front, the core, or the back of the target. The main accelerating mechanisms discussed in this paper are plasma expansion acceleration, where proton acceleration is driven by the hot electron population, and shock acceleration, originating from the laser ponderomotive potential imposed at the front target surface. Three main regimes of proton acceleration are defined and the parameters for which each regime is dominant are obtained. For irradiances close to 1020W∕cm2, the highest proton energies are obtained from thin foils efficiently heated by relativistic transparency. At larger intensities, a complex interplay between collisionless shock acceleration and plasma expansion acceleration is evidenced.

Ion acceleration resulting from the interaction of 11 fs laser pulses of 35 mJ energy with ultrahigh contrast (<10−10) and 1019 W cm−2 peak intensity with foil targets made of various materials and thicknesses at normal (0°) and 45° laser incidence is investigated. The maximum energy of the protons reached ∼1.4 MeV accelerated in the laser propagation direction and ∼1.2 MeV in the opposite direction from a formvar target. The energy conversion efficiency from the laser to the proton beam is estimated to be as high as ∼1.4% at 45° laser incidence using a 51 nm thick target. The high laser contrast indicates the predominance of vacuum heating via Brunel’s effect as an absorption mechanism involving a tiny pre-plasma at the target front. The experimental results are in reasonable agreement with theoretical estimates, where proton acceleration from the target front side in the backward direction is well explained by the Coulomb explosion of a charged cavity formed in a tiny pre-plasma, while forward proton acceleration is likely to be a two-step process: protons are first accelerated in the target front-side cavity and then further boosted in energy through the target back side via the target normal sheath acceleration (TNSA) mechanism.

Proton emission from solid foil targets irradiated by relativistically intense femtosecond laser pulses is studied experimentally. Broad plateaus in energy spectra are measured from micron-thick targets when the incident laser pulses have relatively low intensity contrasts. It is proposed that such proton spectra can be attributed to the combined processes of laser-driven collisionless shock acceleration and target normal sheath acceleration. Simple analytic estimation and two-dimensional particle-in-cell simulations are performed, which support our interpretation. The obtained plateau-shape spectrum may also serve as an effective tool to diagnose the plasma state and verify the ion acceleration mechanisms in laser-solid interactions.

Ion acceleration resulting from the interaction of ultra-high intensity and ultra-high contrast (∼10−10) laser pulses with thin Al foil targets at 30° angle of laser incidence is studied. Proton maximum energies of 30 and 18 MeV are measured along the target normal rear and front sides, respectively, showing intensity scaling as Ib. For the target front bfront= 0.5–0.6 and for the target rear brear= 0.7–0.8 is observed in the intensity range 1020–1021 W/cm2. The fast scaling from the target rear ∼I0.75 can be attributed enhancement of laser energy absorption as already observed at relatively low intensities. The backward acceleration of the front side protons with intensity scaling as ∼I0.5 can be attributed to the to the formation of a positively charged cavity at the target front via ponderomotive displacement of the target electrons at the interaction of relativistic intense laser pulses with a solid target. The experimental results are in a good agreement with theoretical predictions.

Laser-driven particle acceleration has been under intense investigation for the last decade and is of particular interest for key applications such as medical physics, fast ignition and inertial confinement fusion. The dominant ion acceleration mechanism is known as target normal sheath acceleration (TNSA); although easy accessible it suffers from a low energy conversion efficiency. Recently reported maximum ion energies1 are in the range of a few tens of MeV, which is well below the energies needed for most applications. Recently proposed acceleration mechanisms utilize ultra-high contrast laser pulses and ultra-thin solid targets allowing for generation of ions in the GeV range from intense laser-plasma interaction. A high laser contrast suppresses pre-ionization of the solid target by any pre-pulses or laser pedestals and in theory enables acceleration beyond TNSA in regimes such as the break-out afterburner (BOA)2 or radiation pressure acceleration (RPA).

We investigate laser-driven proton acceleration using state-of-the-art multi-petawatt laser technology and a double-layer target design. The front layer is composed of homogenised near-critical density carbon, which enhances the laser pulse through relativistic self-focusing, effectively acting as a lensing medium. This layer is paired with a solid plastic rear layer that serves as the primary acceleration medium. The thicknesses of both layers and the density of the front layer are optimised to maximise acceleration efficiency of the solid layer protons. These protons are accelerated up to 550 MeV through a synergistic interplay of acceleration mechanisms, with hole boring and light sail radiation pressure acceleration playing dominant roles. These mechanisms are further enhanced by target normal sheath acceleration, which benefits from increased laser-to-electron coupling, especially in the front near critical density part. Additionally, proton acceleration is accompanied by the generation of gamma-ray radiation via nonlinear inverse Compton scattering. Our investigation employs fully resolved 3D particle-in-cell simulations, providing comprehensive insights into the underlying dynamics. Detailed technical aspects of the simulation setup are discussed.

Laser-plasma proton acceleration was investigated in the target normal sheath acceleration regime with a target composed of a gas layer and a thin foil. The laser’s shape, duration, energy and frequency are modified as it propagates in the gas, altering the laser-solid interaction leading to proton acceleration. The modified properties of the laser were assessed by both numerical simulations and by measurements. The 3D particle-in-cell simulations have shown that a nearly seven-fold increase in peak intensity at the foil plane is possible. In the experiment, maximum proton energies showed high dependence on the energy transmission of the laser through the gas and a lesser dependence on the size and shape of the pulse. At high gas densities, where high intensity was expected, laser energy depletion and pulse distortion suppressed proton energies. At low densities, with the laser focused far behind the foil, self-focusing was observed and the gas showed a positive effect on proton energies. The promising results of this first exploration motivate further study of the target.

We present experimental results obtained at the CELIA laboratory using the laser ECLIPSE to study proton acceleration from ultra-intense laser pulses. Several types of targets were irradiated with different laser conditions (focusing and prepulse level). Proton emission was characterized using time-of-flight detectors (SiC and diamond) and a Thomson parabola spectrometer. In all cases, the maximum energy of observed protons was of the order of 260 keV with a large energy spectrum. Such characteristics are typical of protons emitted following the target normal sheath acceleration mechanism for low-energy short-pulse lasers like ECLIPSE.

Some applications of fast ions driven by a short (⩽1 ps) laser pulse (e.g. fast ignition of ICF targets, x-ray laser pumping, laboratory astrophysics research or some nuclear physics experiments) require ion beams of picosecond (or shorter) time durations and of very high ion current densities (∼1010 A cm−2 or higher). A possible way of producing ion beams with such extreme parameters is ballistic focusing of fast ions generated by a target normal sheath acceleration (TNSA) mechanism at relativistic laser intensities. In this paper we discuss another method, where the production of short-pulse ion beams of ultrahigh current densities is possible in a planar geometry at subrelativistic laser intensities and at a low energy (⩽1 J) of the laser pulse. This method—referred to as skin-layer ponderomotive acceleration (S-LPA)—uses strong ponderomotive forces induced at the skin-layer interaction of a short laser pulse with a proper preplasma layer in front of a solid target. The basic features of the high-current ion generation by S-LPA were investigated using a simplified theory, numerical hydrodynamic simulations and measurements. The experiments were performed with subjoule 1 ps laser pulses interacting with massive or thin foil targets at intensities of up to 2 × 1017 W cm−2. It was found that both in the backward and forward directions highly collimated high-density ion beams (plasma blocks) with current densities at the ion source (close to the target) approaching 1010 A cm−2 are produced, in accordance with the theory and numerical calculations. These ion current densities were found to be comparable to (or even higher than) those estimated from recent short-pulse TNSA experiments with relativistic laser intensities. Apart from the simpler physics of the laser–plasma interaction, the advantage of the considered method is the low energy of the driving laser pulses allowing the production of ultrahigh-current-density ion beams with a high repetition rate. It opens a prospect for unique tabletop experiments in various fields of physical and technological research.

Advances in laser technology have led to ever-increasing laser intensities. As a result, in addition to the amplified spontaneous emission and pedestal, it has become necessary to accurately treat the relativistic rising edge component. This component has not needed much consideration in the past because of its not relativistic intensity. In the previous study, a thin contamination layer was blown away from the target by the rear sheath field due to the relativistic rising edge component, and the target bulk was accelerated by the sheath field due to the main pulse. These indicated that the proton acceleration is not efficient in the target normal sheath acceleration by the ultrahigh intense femtosecond laser if the proton-containing layer is as thin as the contamination layer. Here we employ a double-layer target, making the second (rear) layer thick enough not to be blown away by the rising edge, so that the second layer is accelerated by the main pulse. The first layer is composed of heavy ions to reduce the total thickness of the target for efficient proton acceleration. We investigate an optimal design of a double-layer target for proton acceleration by the ultrahigh intense femtosecond laser considering the relativistic rising edge using two-dimensional particle-in-cell simulations. We also discuss how to optimize the design of such a double-layer target and find that it can be designed with two conditions: the first layer is not penetrated by hole boring, and the second layer is not blown away by the rising edge.

The discovery that ultra-intense laser pulses (I > 1018 W/cm2) can produce short pulse, high energy proton beams has renewed interest in the fundamental mechanisms that govern particle acceleration from laser-solid interactions. Experiments have shown that protons present as hydrocarbon contaminants on laser targets can be accelerated up to energies > 50 MeV. Different theoretical models that explain the observed results have been proposed. One model describes a front-surface acceleration mechanism based on the ponderomotive potential of the laser pulse. At high intensities (I > 1018 W/cm2), the quiver energy of an electron oscillating in the electric field of the laser pulse exceeds the electron rest mass, requiring the consideration of relativistic effects. The relativistically correct ponderomotive potential is given by Up = ([1 + Iλ2/1.3 x 1018]1/2 - 1) m{sub o}c2, where Iλ2 is the irradiance in W μm2/cm2 and moc2 is the electron rest mass. At laser irradiance of Iλ2 ~ 1020 W μm2/cm2, the ponderomotive potential can be of order several MeV. A few recent experiments--discussed in Chapter 3 of this thesis--consider this ponderomotive potential sufficiently strong to accelerate protons from the front surface of the target to energies up to tens of MeV. Another model, known as Target Normal Sheath Acceleration (TNSA), describes the mechanism as an electrostatic sheath on the back surface of the laser target. According to the TNSA model, relativistic hot electrons created at the laser-solid interaction penetrate the foil where a few escape to infinity. The remaining hot electrons are retained by the target potential and establish an electrostatic sheath on the back surface of the target. In this thesis we present several experiments that study the accelerated ions by affecting the contamination layer from which they originate. Radiative heating was employed as a method of removing contamination from palladium targets doped with deuterium. We present evidence that ions heavier than protons can be accelerated if hydrogenous contaminants that cover the laser target can be removed. We show that deuterons can be accelerated from the deuterated-palladium target, which has been radiatively heated to remove contaminants. Impinging a deuteron beam onto a tritiated-titanium catcher could lead to the development of a table-top source of short-pulse, 14-MeV fusion neutrons. We also show that by using an argon-ion sputter gun, contaminants from one side of the laser target can be selectively removed without affecting the other side. We show that irradiating a thin metallic foil with an ultra-intense laser pulse produces a proton beam with a yield of 1.5-2.5 1011 and temperature, kT = 1.5 MeV with a maximum proton energy > 9 MeV. Removing contaminants from the front surface of the laser target with an argon-ion sputter gun, had no observable effect on the proton beam. However, removing contaminants from the back surface of the laser target reduced the proton beam by two orders of magnitude to, at most, a yield of ~ 109 and a maximum proton energy < 4 MeV. Based on these observations, we conclude that the majority (> 99%) of high energy protons (E > 5 MeV) from the interaction of an ultra-intense laser pulse with a thin foil originate on the back surface of the foil--as predicted by the TNSA model. Our experimental results are in agreement with PIC simulations showing back surface protons reach energies up to 13 MeV, while front surface protons reach a maximum energy of 4 MeV. Well diagnosed and controllable proton beams will have many applications: neutron radiography, material damage studies, production of medical isotopes, and as a high-resolution radiography tool for diagnosing opaque materials and plasmas. Well collimated and focusable ion beams may also prove beneficial for alternative inertial-fusion concepts such as proton fast ignition, a potentially viable method for achieving a controlled fusion reaction in the laboratory earlier than expected.

Target normal sheath acceleration (TNSA) is a method employed in laser–matter interaction experiments to accelerate light ions (usually protons). Laser setups with durations of a few 10 fs and relatively low intensity contrasts observe plateau regions in their ion energy spectra when shooting on thin foil targets with thicknesses of the order of 10 μm. In this paper, we identify a mechanism which explains this phenomenon using one-dimensional particle-in-cell simulations. Fast electrons generated from the laser interaction recirculate back and forth through the target, giving rise to time-oscillating charge and current densities at the target backside. Periodic decreases in the electron density lead to transient disruptions of the TNSA sheath field: peaks in the ion spectra form as a result, which are then spread in energy from a modified potential driven by further electron recirculation. The ratio between the laser pulse duration and the recirculation period (dependent on the target thickness, including the portion of the pre-plasma which is denser than the critical density) determines if a plateau forms in the energy spectra.

Laser pre‐pulse is a major issue in experiments on laser‐generation of protons, often limiting the performances of laser sources. In this paper, we show how we can actively use a low intensity prepulse (<1013 W/cm2, ns duration) to manipulate the proton beam direction or spatial energy distribution. The prepulse is focused onto the front surface of a thin foil before the arrival of the high intensity pulse (≈1019 W/cm2, ps duration). Under oblique high‐intensity irradiation and for low prepulse intensities, the proton beam is directed away from the target normal. Deviation is towards the laser forward direction, with an angle that increases with the level and duration of the ASE pedestal. Also, for a given laser pulse, beam deviation increases with proton energy. The observations are discussed in terms of Target Normal Sheath Acceleration, in combination with a laser‐controllable shock wave locally deforming the target surface. Results obtained with an annular intensity distribution of the prepulse show s...

It was recently shown that a promising way to accelerate protons in the forward direction to high energies is to use under-dense or near-critical density targets instead of solids. Simulations have revealed that the acceleration process depends on the density gradients of the plasma target. Indeed, under certain conditions, the most energetic protons are predicted to be accelerated by a collisionless shock mechanism that significantly increases their energy. We report here the results of a recent experiment dedicated to the study of longitudinal ion acceleration in partially exploded foils using a high intensity (∼5 × 1018 W/cm2) picosecond laser pulse. We show that protons accelerated using targets having moderate front and rear plasma gradients (up to ∼8 μm gradient length) exhibit similar maximum proton energy and number compared to proton beams that are produced, in similar laser conditions, from solid targets, in the well-known target normal sheath acceleration regime. Particle-In-Cell simulations, performed in the same conditions as the experiment and consistent with the measurements, allow laying a path for further improvement of this acceleration scheme.