Supraclassical measurement using single-atom control of an atomic ensemble

Until very recently a single atom interacting with an electromagnetic field could only be a topic of theoretical consideration because experimentally only ensembles of atoms were accessible. Atomic spectra and the probabilities of transitions in atoms had been successfully studied in atomic ensembles for a long time. Quantum mechanics enables one to calculate both spectra and probabilities. However, quantum mechanics predicts that any transition happens at a random moment of time. In accordance with this prediction a single atom irradiated by light will make random jumps between its ground and excited electronic states. However, these jumps cannot be observed if we detect emission from the whole atomic ensemble, because a statistical average hides the random character of the processes. Therefore they cannot be observed in ensembles. This is only one example of new aspects which emerge when we move from atomic ensembles to a single atom. In this book we intend to discuss not only problems of probabilistic and spectral calculations, but also various random characteristics of atoms and molecules, the so-called quantum trajectories, which are typical in the spectroscopy of single atoms or molecules. In order to prepare for the discussion of quantum trajectories, we have to discuss the basic principles underlying the spectroscopy of a single two-level atom interacting with a transverse electromagnetic field.

We propose a nonadiabatic non-Abelian geometric quantum operation scheme to realize universal quantum computation with mesoscopic Rydberg atoms. A single control atom entangles a mesoscopic ensemble of target atoms through long-range interactions between Rydberg states. We demonstrate theoretically that both the single qubit and two-qubit quantum gates can achieve high fidelities around or above 99.9% in ideal situations. Besides, to address the experimental issue of Rabi frequency fluctuation (Rabi error) in Rydberg atom and ensemble, we apply the dynamical-invariant-based zero systematic-error sensitivity (ZSS) optimal control theory to the proposed scheme. Our numerical simulations show that the average fidelity could be 99.98% for single ensemble qubit gate and 99.94% for two-qubit gate even when the Rabi frequency of the gate laser acquires 10% fluctuations. We also find that the optimized scheme can also reduce errors caused by higher-order perturbation terms in deriving the Hamiltonian of the ensemble atoms. To address the experimental issue of decoherence error between the ground state and Rydberg levels in Rydberg ensemble, we introduce a dispersive coupling regime between Rydberg and ground levels, based on which the Rydberg state is adiabatically discarded. The numerical simulation demonstrate that the quantum gate is enhanced. By combining strong Rydberg atom interactions, nonadiabatic geometric quantum computation, dynamical invariant and optimal control theory together, our scheme shows a new route to construct fast and robust quantum gates with mesoscopic atomic ensembles. Our study contributes to the ongoing effort in developing quantum information processing with Rydberg atoms trapped in optical lattices or tweezer arrays.

Quantum gates are fundamental in Quantum computing for their role in manipulating elementary information carriers referred to as quantum bits. In this paper, a theoretical scheme for realizing a quantum Hadamard and a quantum controlled-NOT logic gates operations in the anti-Jaynes-Cummings interaction process is provided. Standard Hadamard operation for a specified initial atomic state is achieved by setting a specific sum frequency and photon number in the normalized anti-Jaynes-Cummings qubit state transition operation with the interaction component of the anti-Jaynes-Cummings Hamiltonian generating the state transitions. The quantum controlled-NOT logic gate is realized when a single atomic qubit defined in a two-dimensional Hilbert space is the control qubit and two non-degenerate and orthogonal polarized cavities defined in a two-dimensional Hilbert space make the target qubit. With precise choice of interaction time in the anti-Jaynes-Cummings qubit state transition operations defined in the anti-Jaynes-Cummings sub-space spanned by normalized but non-orthogonal basic qubit state vectors, ideal unit probabilities of success in the quantum controlled-NOT operations is determined.

Universal quantum computing relies on high-fidelity entangling operations. Here, we demonstrate that four coupled qubits can operate as a quantum gate, where two qubits control the operation on two target qubits (a four-qubit gate). This configuration can implement four different controlled two-qubit gates: two different entangling swap and phase operations, a phase operation distinguishing states of different parity, and the identity operation (idle quantum gate), where the choice of gate is set by the state of the control qubits. The device exploits quantum interference to control the operation on the target qubits by coupling them to each other via the control qubits. By connecting several four-qubit devices in a two-dimensional lattice, one can achieve a highly connected quantum computer. We consider an implementation of the four-qubit gate with superconducting qubits, using capacitively coupled qubits arranged in a diamond-shaped architecture.

A brief overview of the current state of the experimental research on the development of the element base of quantum computers with qubits based on single neutral atoms trapped in optical traps. The requirements for qubits, peculiarities of single neutral atoms as qubits, methods for the quantum register development and for the implementation of single-qubit quantum logic operations in the laser and microwave fields, and two-qubit operations through the dipole–dipole interaction after a short laser excitation of atoms to the Rydberg states are discussed. The results of the experiments on the observation of the interaction of two Rydberg atoms at a Forster resonance controlled by the dc and radio-frequency electric field are presented.

The qubit state is represented by a coherent superposition of its orthonormal basis states (|0〉 and |1〉). The probability distribution of a qubit is a discrete probability distribution of the qubits probability amplitudes. Setting a custom probability amplitudes allows a qubit to evolve to any desired state. In this paper a controlled n-root of X gate is simulated on a real quantum processor using IBMs Quantum Experience platform. A custom quantum gate could be constructed where the only inputs are the control and target qubits and the desired probability distribution for the target qubit.

A single atom is the prototypical quantum system, and a natural candidate for a quantum bit, or qubit--the elementary unit of a quantum computer. Atoms have been successfully used to store and process quantum information in electromagnetic traps, as well as in diamond through the use of the nitrogen-vacancy-centre point defect. Solid-state electrical devices possess great potential to scale up such demonstrations from few-qubit control to larger-scale quantum processors. Coherent control of spin qubits has been achieved in lithographically defined double quantum dots in both GaAs (refs 3-5) and Si (ref. 6). However, it is a formidable challenge to combine the electrical measurement capabilities of engineered nanostructures with the benefits inherent in atomic spin qubits. Here we demonstrate the coherent manipulation of an individual electron spin qubit bound to a phosphorus donor atom in natural silicon, measured electrically via single-shot read-out. We use electron spin resonance to drive Rabi oscillations, and a Hahn echo pulse sequence reveals a spin coherence time exceeding 200 µs. This time should be even longer in isotopically enriched (28)Si samples. Combined with a device architecture that is compatible with modern integrated circuit technology, the electron spin of a single phosphorus atom in silicon should be an excellent platform on which to build a scalable quantum computer.

Non-adiabatic holonomic quantum gate in decoherence-free subspaces is of greatly practical importance due to its built-in fault tolerance, coherence stabilization virtues, and short run-time. Here, we propose some compact schemes to implement two- and three-qubit controlled unitary quantum gates and Fredkin gate. For the controlled unitary quantum gates, the unitary operator acting on the target qubit is an arbitrary single-qubit gate operation. The controlled quantum gates can be directly implemented by utilizing non-adiabatic holonomy in decoherence-free subspaces and the required resource for the decoherence-free subspace encoding is minimal by using only two neighboring physical qubits undergoing collective dephasing to encode a logical qubit.

Preparation of W state among spatially separated atomic ensembles collectively controlled by a single atom via adiabatic passage

Based on a quantum analysis of two capacitively coupled current-biased Josephson junctions, we propose two fundamental two-qubit quantum logic gates. Each of these gates, when supplemented by single-qubit operations, is sufficient for universal quantum computation. Numerical solutions of the time-dependent Schrödinger equation demonstrate that these operations can be performed with good fidelity.

Ultra-cold atoms are highly sensitive to both inertial effects and electromagnetic fields, making atom interferometers excellent candidates for a variety of precision sensing applications. Furthermore, highly tunable atomic interactions combined with well established experimental techniques for trapping, cooling and manipulating ensembles of ultra-cold atoms, make them well suited to quantum enhancement. For these reasons, ensembles of ultra-cold atoms are excellent candidates for quantum-enhanced measurement devices. Broadly, this thesis presents a number of theoretical results which share the aim of progressing the proof-of-principle regime of current experiments to genuinely useful, ultra-precise quantum enhanced sensors.In Chapter 4 we explore the challenge of devising a useful, quantum-enhanced inertial measurement - to date no such experiment has been performed. Specifically, we present a model of a spin-squeezed rotation sensor utilising the Sagnac effect in a spin-1 Bose-Einstein condensate in a ring trap. The two input states for the interferometer are seeded using Raman pulses with Laguerre-Gauss beams and are amplified by the bosonic enhancement of spin-exchange collisions, resulting in spin-squeezing and potential quantum enhancement in the interferometry. The ring geometry has an advantage over separated beam path atomic rotation sensors due to the uniform condensate density. We model the interferometer both analytically and numerically for realistic experimental parameters and find that significant quantum enhancement is possible. However, this enhancement is partially degraded when working in a regime with strong atomic interactions, indicating that perhaps interaction-based squeezing is not the best route to a quantum-enhanced inertial measurement.Continuing the theme of practical spin-squeezing with atomic interactions, in Chapter 5 we explore methods to combat detection noise, which is currently one of the most significant experimental limitations for quantum-enhanced atom interferometers. A useful quantum-enhanced interferometer requires nonclassical states with a high particle number and the (close to) optimal exploitation of the states' quantum correlations. Unfortunately, the single-particle detection resolution demanded by conventional protocols, such as spin squeezing via one-axis twisting, places severe limits on the particle number. Additionally, the challenge of finding optimal measurements (that saturate the quantum Cram´er-Rao bound) for an arbitrary nonclassical state limits most metrological protocols to only moderate levels of quantum enhancement. “Interaction-based readout” protocols have been shown to allow optimal interferometry or to provide robustness against detection noise at the expense of optimality. We prove that one has great flexibility in constructing an optimal protocol, thereby allowing it to also be robust to detection noise. This requires the full probability distribution of outcomes in an optimal measurement basis, which is typically easily-accessible and can be determined from specific criteria we provide. Additionally, we quantify the robustness of several classes of interaction-based readouts under realistic experimental constraints. We determine that optimal and robust quantum metrology is achievable in current spin-squeezing experiments.Macroscopic superposition states (known as spin-cat states in atomic ensembles) achieve the ultimate quantum precision limit. In Chapters 6 and 7 we turn our attention to studying decoherence that arises in creating and manipulating these states. In its simplest form, decoherence occurs when a quantum state is entangled with a second state, but the results of measurements made on the second state are not accessible. As the second state has effectively ``measured the first, in Chapter 6 we argue that the quantum Fisher information is the relevant metric for predicting and quantifying this kind of decoherence. In particular we apply this analysis to studying decoherence imparted on spin-cat states via atom-light interactions, which are an essential process in atom interferometry. We find that, compared to classical atomic states, spin-cat states are highly susceptible to this kind of decoherence. We investigate the required optical field occupation, such that this decoherence is negligible.Finally, in Chapter 7 we explore the deleterious effects of spatial and phase dynamics during the creation of spin-cat states via one-axis twisting in a two-component Bose-Einstein condensate. We simulate the breathing dynamics in 1 spatial dimension, employing the method of Sinatra and Castin, whereby the state is expanded into the Fock basis, with each basis state evolving within the Hartree-Fock approximation. This method is able to capture both multi-mode effects and quantum correlations, which allows us to calculate the quantum Fisher information. We find that so long as the time taken for the condensate to reach a spin-cat state is an integer multiple of the breathing period, it is sometimes possible to realise something extremely close to a spin-cat state, despite significant dynamics. These results indicate that large non-linearities, and the associated speed-up in entangling dynamics, are not fundamentally incompatible with the production of fragile, highly entangled states such as spin-cat states.

High-fidelity single- and multiqubit operations compose the backbone of quantum information processing. This fidelity is based on the ability to couple single- or two-qubit levels in an extremely coherent and precise manner. A necessary condition for coherent quantum evolution is a highly stable local oscillator driving these transitions. Here we study the effect of fast noise, that is, noise at frequencies much higher than the local oscillator linewidth, on the fidelity of one- and two-qubit gates in a trapped-ion system. We analyze and measure the effect of fast noise on single-qubit operations, including resonant $\ensuremath{\pi}$ rotations and off-resonant sideband transitions. We further numerically analyze the effect of fast phase noise on the M\o{}lmer-S\o{}rensen two-qubit gate. We find a unified and simple way to estimate the performance of all of these operations through a single parameter given by the noise power spectral density at the qubit response frequency. While our analysis focuses on phase noise and on trapped-ion systems, it is relevant for other sources of fast noise as well as for other qubit systems in which spinlike qubits are coupled by a common bosonic field. Our analysis can help in guiding the design of quantum hardware platforms and gates, improving their fidelity towards fault-tolerant quantum computing.

Resonant transverse driving of a two-level system as viewed in the rotating frame couples two degenerate states at the Rabi frequency, an amazing equivalence that emerges in quantum mechanics. While spectacularly successful at controlling natural and artificial quantum systems, certain limitations may arise (e.g., the achievable gate speed) due to non-idealities like the counter-rotating term. Here, we explore a complementary approach to quantum control based on non-resonant, non-adiabatic driving of a longitudinal parameter in the presence of a fixed transverse coupling. We introduce a superconducting composite qubit (CQB), formed from two capacitively coupled transmon qubits, which features a small avoided crossing -- smaller than the environmental temperature -- between two energy levels. We control this low-frequency CQB using solely baseband pulses, non-adiabatic transitions, and coherent Landau-Zener interference to achieve fast, high-fidelity, single-qubit operations with Clifford fidelities exceeding $99.7\%$. We also perform coupled qubit operations between two low-frequency CQBs. This work demonstrates that universal non-adiabatic control of low-frequency qubits is feasible using solely baseband pulses.

Quantum controlled-phase-flip (CPF) gate between a flying photon qubit and a stationary atomic qubit could allow the linking of distant computational nodes in a quantum network. Here we present a scheme to realize quantum CPF gate between a flying optical photon and an atomic ensemble based on cavity input-output process and Rydberg blockade. When a flying single-photon pulse is reflected off the cavity containing a Rydberg atomic ensemble, the dark resonance and Rydberg blockade induce a conditional phase shift for the photon pulse, thus we can achieve the CPF gate between the photon and the atomic ensemble. Assisted by Rydberg blockade interaction, our scheme works in the N-atoms strong-coupling regime and significantly relaxes the requirement of strong coupling of single atom to photon in the optical cavity.

Preparation of multi-party entanglement of individual photons and atomic ensembles