- Research Article
18
- 10.1364/josab.35.002754
Computational analysis of dispersive and nonlinear 2D materials by using a GS-FDTD method
- Oct 11, 2018
- Journal of the Optical Society of America B
- Jian Wei You + 3 more +3
In this paper, we propose a novel numerical method for modeling\nnanostructures containing dispersive and nonlinear two-dimensional (2D)\nmaterials, by incorporating a nonlinear generalized source (GS) into the\nfinite-difference time-domain (FDTD) method. Starting from the expressions of\nnonlinear currents characterizing nonlinear processes in 2D materials, such as\nsecond- and third-harmonic generation, we prove that the nonlinear response of\nsuch nanostructures can be rigorously determined using two linear simulations.\nIn the first simulation, one computes the linear response of the system upon\nits excitation by a pulsed incoming wave, whereas in the second one the system\nis excited by a nonlinear generalized source, which is determined by the linear\nnear-field calculated in the first linear simulation. This new method is\nparticularly suitable for the analysis of dispersive and nonlinear 2D\nmaterials, such as graphene and transition-metal dichalcogenides, chiefly\nbecause, unlike the case of most alternative approaches, it does not require\nthe thickness of the 2D material. In order to investigate the accuracy of the\nproposed GS-FDTD method and illustrate its versatility, the linear and\nnonlinear response of graphene gratings have been calculated and compared to\nresults obtained using alternative methods. Importantly, the proposed GS-FDTD\ncan be extended to 3D bulk nonlinearities, rendering it a powerful tool for the\ndesign and analysis of more complicated nanodevices.\n
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