UMI MajuLab

Optical control offers a non-contact, high-precision and ultrafast route to manipulating quantum material properties1-5. Fractional Chern ferromagnetic states in moiré superlattices are apromisingplatform by whichto pursue topological quantum computing6-10, but an effective optical control protocol has remained elusive. Here we demonstrate robust optical switching of integer and fractional Chern ferromagnets in twisted molybdenum ditelluride (MoTe2) bilayers using continuous-wave circularly polarized light. Highly efficient optical manipulation of spin orientations in the topological ferromagnet regime is realized at zero field using a pump light power as low as 28 nW µm-2. Using this optically induced transition, we also demonstrate magnetic bistate cycling and spatially resolved writing of ferromagnetic domain walls. This work establishes a reliable and efficient optical control scheme for moiré Chern ferromagnets, paving the way for dissipationless spintronics and quantized Chern junction devices.

Abstract Excitonics is an emerging field focused on exploiting and manipulating excitons generated through light-matter interactions. Advancing the field into X-ray excitonics requires precise energy and time control of core-exciton resonances, enabling non-linear X-ray phenomena such as element-specific X-ray transient gratings, and advancing material characterization. To achieve these objectives, it is essential to comprehend the role of many-body effects governing core-exciton dynamics. In this work, we address this challenge by combining experiments with an ab initio approach specifically developed to interpret pump-probe excitations. Applied to the prototypical wide-bandgap semiconductor ZnO, first-principles calculations reproduce experimental results and unveil how the density and distribution of photoexcited carriers dynamically tune Coulomb screening, thereby controlling core-exciton binding energies, while Pauli blocking remains negligible. These insights inform a method for dynamically controlling core-exciton resonances at absorption edges, achieving either a uniform spectral blue shift caused by thermalized carrier distributions on picosecond timescales, or distinct blue shifts for individual resonances, driven by time-dependent carrier distributions on femtosecond timescales.

So far, exciton-polariton (polariton) lasers were mostly single-mode lasers based on microcavities. Despite the large repulsive polariton-polariton interaction, a pulsed mode-locked polariton laser was never, to our knowledge, reported. Here, we use a 60-µm-long GaN-based waveguide surrounded by distributed Bragg reflectors forming a multi-mode horizontal cavity. We demonstrate experimentally and theoretically a polariton mode-locked micro-laser operating in the blue-UV, at room temperature, with a 300 GHz repetition rate and 100-fs-long pulses. The mode-locking is demonstrated by the compensation (linearization) of the mode dispersion by the self-phase modulation induced by the polariton-polariton interaction. It is also supported by the observation in experiment and theory of the typical envelope frequency profile of a bright soliton.

We study the time evolution of mean values of quantum operators in a regime plagued by two difficulties: the smallness of ℏ and the presence of strong and ubiquitous classical chaos. While numerics become too computationally expensive for purely quantum calculations as ℏ→0, methods that take advantage of the smallness of ℏ-that is, semiclassical methods-suffer from both conceptual and practical difficulties in the deep chaotic regime. We implement an approach which addresses these conceptual problems, leading to a deeper understanding of the origin of the interference contributions to the operator's mean value. We show that in the deep chaotic regime our approach is capable of unprecedented accuracy, while a standard semiclassical method (the Herman-Kluk propagator) produces only numerical noise. Our work paves the way to the development and employment of more efficient and accurate methods for quantum simulations of systems with strongly chaotic classical limits.

Measuring an observable which does not commute with the Hamiltonian of a quantum system usually modifies the mean energy of this system. In an autonomous measurement scheme, coupling the system to a quantum meter, the system's energy change must be compensated by the meter's energy change. Here, we theoretically study such an autonomous meter-system dynamics: a qubit interacting dispersively with a light pulse propagating in a one-dimensional waveguide. The phase of the light pulse is shifted, conditioned to the qubit's state along the z-direction, while the orientation of the qubit Hamiltonian is arbitrary. As the interaction is dispersive, photon number is conserved so that energy balance has to be attained by spectral deformations of the light pulse. Building on analytical and numerical solutions, we reveal the mechanism underlying this spectral deformation and display how it compensates for the qubit's energy change. We explain the formation of a three-peak structure of the output spectrum and we provide the conditions under which this is observable.

Ramsey interferometry is an important technique in precision spectroscopy and quantum coherence measurement. The authors explore an innovative scheme in which splitter pulses are implemented by geometrical means, eliminating the temporal dependence of the atom-light interaction. This translates to an interferometer that is insensitive to the mean velocity of the atomic ensemble, making it suitable for applications in quantum computing and simulation, as well as atomtronic circuits. Using this geometric Ramsey interferometer, the team measures the phase accumulation during the free-evolution time due to a geometric scalar term.

Self-oscillations are the result of an efficient mechanism generating periodic motion from a constant power source. In quantum devices, these oscillations may arise due to the interaction between single electron dynamics and mechanical motion. We show that, due to the complexity of this mechanism, these self-oscillations may irrupt, vanish, or exhibit a bistable behavior causing hysteresis cycles. We observe these hysteresis cycles and characterize the stability of different regimes in both single- and double-quantum-dot configurations. In particular cases, we find these oscillations stable for over 20 s, many orders of magnitude above electronic and mechanical characteristic timescales, revealing the robustness of the mechanism at play. Published by the American Physical Society 2024

A form of quantum control is proposed by applying twisted light, also known as optical vortex beams, to drive ultranarrow atomic transitions in neutral Ca, Mg, Yb, Sr, Hg, and Cd bosonic isotopes. This innovative all-optical spectroscopic method introduces spatially tailored electric and magnetic fields to fully rewrite atomic selection rules, reducing simultaneously probe-induced frequency shifts and additional action of external ac and dc field distortions. A twisted-light focused probe beam produces strong longitudinal electric and magnetic fields along the laser propagation axis, which opens the $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{0}$ doubly forbidden clock transition with a high $E1M1$ two-photon excitation rate. This long-lived clock transition is thus immune to nonscalar electromagnetic perturbations. Zeeman components of the $M2$ magnetic quadrupole $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{2}$ transition considered for quantum computation and simulation are now selectively driven by transverse or longitudinal field gradients with vanishing electric fields. These field gradients are manipulated by the mutual action of orbital and spin angular momentum of the light beam and are used in presence of tunable vector and tensor polarizabilities. A combination of these two different twisted-light induced clock transitions within a single quantum system, at the same magic wavelength and in presence of a common thermal environment, significantly reduces systematic uncertainties. Furthermore, it generates an optical synthetic frequency which efficiently limits the blackbody radiation shift and its variations at room temperature. Engineering light-matter interaction by optical vortices merged with composite pulses will ultimately benefit experimental atomic and molecular platforms targeting an optimal coherent control of quantum states, reliant quantum simulation, novel approaches to atomic interferometry, and precision tests of fundamental theories in physics and high-accuracy optical metrology.

Ramsey interferometry is a key technique for precision spectroscopy and to probe the coherence of quantum systems. Typically, an interferometer is constructed using two quantum states and involves a time-dependent interaction with two short resonant electromagnetic pulses. Here, we explore a different type of Ramsey interferometer where we perform quantum state manipulations by geometrical means, eliminating the temporal dependence of the interaction. We use a resonant tripod scheme in ultracold strontium atoms where the interferometric operation is restricted to a two-dimensional dark-state subspace in the dressed-state picture. The observed interferometric phase accumulation is due to an effective geometric scalar term in the dark-state subspace, which remarkably does not vanish during the free evolution time when the light-matter interaction is turned off. This study opens the door for more robust interferometers operating on multiple input-output ports.

Experiments in cold atom systems see almost identical signatures of many body
\nlocalization (MBL) in both one-dimensional ($d=1$) and two-dimensional ($d=2$)
\nsystems despite the thermal avalanche hypothesis showing that the MBL phase is
\nunstable for $d>1$. Underpinning the thermal avalanche argument is the
\nassumption of exponential localization of local integrals of motion (LIOMs). In
\nthis work we demonstrate that addition of a confining potential -- as is
\ntypical in experimental setups -- allows a non-interacting disordered system to
\nhave super-exponentially (Gaussian) localized wavefunctions, and an interacting
\ndisordered system to undergo a localization transition. Moreover, we show that
\nGaussian localization of MBL LIOMs shifts the quantum avalanche critical
\ndimension from $d=1$ to $d=2$, potentially bridging the divide between the
\nexperimental demonstrations of MBL in these systems and existing theoretical
\narguments that claim that such demonstrations are impossible.