Single photon frequency up-conversion and its applications

This thesis covers the development and the characterization of a single photon detector based on a superconducting microcalorimeter. The detector development is motivated by the Any Light Particle Search II (ALPS II) experiment at DESY in Hamburg, which searches for weakly interacting sub-eV particles (WISPs). There- fore, a detection of low-fluxes of 1064 nm light is required. The work is divided in three analyses: the characterization of a milli-kelvin (mK) cryostat, the character- ization of superconducting sensors for single photon detection, and the determina- tion of dark count rates concerning 1064 nm signals. Firstly, an adiabatic demagnetization refrigerator (ADR) is characterized, which allows to reach mK-temperatures. During commissioning, the ADR cryostat is op- timized and prepared to stably cool superconducting sensors at 80 mK 25 K. It is found that sensors can be continuously operated for 20 h before recharging the system in < 2 h. Furthermore, the adiabatic system reaches a chance of success of 80 % for a recharge without technical problems. Secondly, superconducting sensors are analyzed. The focus is on microcalori- metric transition-edge sensors (TESs) based on 20 nm Tungsten (W) films fabri- cated by the U.S. National Institute of Standards and Technology (NIST). NIST TESs have a near unity detection e ciency for 1064 nm light (literature value). The energy resolution for 1064 nm signals is measured to be < 8 %. The expo- nential falling time of a photon pulse is 1.5 s. Furthermore, by determining TES parameters, it is found that the linear TES theory describes measured photon pulses well. The TES response is read out by a superconducting quantum interference device (SQUID) fabricated by Physikalisch-Technische Bundesanstalt (PTB). The system bandwidth is measured to be 0.9 MHz. Finally, the operation in the ADR cryostat as well as the ALPS II laboratory is optimized. This setup forms the ALPS TES detector. Thirdly, the background is measured to obtain a dark count rate for 1064 nm signals. The ALPS TES detector is calibrated by a 1064 nm single photon source and methods are developed to analyze signals. In long-term measurements, back- ground events are measured by using di erent optical setups. By operating the TES without an optical link outside mK-environment, intrinsic background components are observed and classified. This results in an intrinsic dark count rate for 1064 nm signals of 1 : 0 10

The prototype of a quantum random number generator is a single photon which impinges onto a beam splitter and is then detected by single photon detectors at one of the two output paths. Prior to detection, the photon is in a quantum mechanical superposition state of the two possible outcomes with –ideally– equal amplitudes until its position is determined by measurement. When the two output modes are observed by a single photon detector, the generated clicks can be interpreted as ones and zeros – and a raw random bit stream is obtained. Here we implement such a random bit generator based on single photons from a defect center in diamond. We investigate the single photon emission of the defect center by an anti-bunching measurement. This certifies the “quantumness” of the supplied photonic input state, while the random “decision” is still based on the vacuum fluctuations at the open port of the beam-splitter. Technical limitations, such as intensity fluctuations, mechanical drift, and bias are discussed. A number of ways to suppress such unwanted effects, and an a priori entropy estimation are presented. The single photon nature allows for a characterization of the non-classicality of the source, and allows to determine a background fraction. Due to the NV-center’s superior stability and optical properties, we can operate the generator under ambient conditions around the clock. We present a true 24/7 operation of the implemented random bit generator.

Single photon technology is enabling for quantum communication and processing. Combining single photon sources, routing circuitry and highly efficient detectors in a high yield, low-loss and scalable fashion represent today a major challenge. Nanophotonic devices allow for the realization of on-chip small footprint architectures for generating, manipulating and detecting single photons. Waveguide-integrated superconducting nanowire single photon detectors are today state-of-the art devices capable of detecting single photons propagating in an integrated photonic circuit with high efficiency, speed and low timing uncertainty. Their excellent metrics in the near-infrared allows to directly interface on-chip devices with existing C-Band communication technology systems. To move towards high communication speed, efficient detectors able to sustain Gcps count rate are desirable. Here we present the design process and the experimental characterization of a new generation of fast detectors, consisting of µm-long NbN superconducting nanowires embedded in a SOI two-dimensional photonic crystal cavity. Almost 70% efficiency at telecommunication wavelengths has been achieved with negligible dark counts and sub-ns recovery time, which could enable Gcps count rates.

We describe the simplest single–photon encoding schemes and introduce the concept of a quantum optical gate. These gates can be used to build up arbitrary entangled states of many initially separate single photons. Experimental realization of such a gate involves the development of nonlinear phase shift elements sensitice at the single quantum level. We report our experimental efforts using linear optical elements and non–classical sources where we are able to demonstrate interference and entanglement of initially separate single–photon pulses.

Single-photon frequency upconversion is a nonlinear process where the frequency of the signal photon is translated to the higher frequency with the complete preservation of all the quantum characteristics of the “flying” qubits [1,2]. One promising application of the singlephoton frequency upconversion is converting the infrared photons to the desired spectral regime (usually visible regime) where the high performance detectors are available for sensitive detections [3-6]. The infrared single-photon frequency upconversion detection technique has been successfully used in a variety of applications, including infrared imaging [7] and infrared ultra-sensitive spectroscopy [8,9]. Additionally, such upconversion detector has greatly benefited the applications stringently requiring efficient photon detection in optical quantum computation and communication [10-12]. Furthermore, due to the phase-matching requirement in the frequency upconversion process, the upconversion detectors have some unique features, such as narrow-band wavelength acceptance [13] and polarization sensitivity [14], both of which render them very useful for fiber based quantum systems [15]. In the recent decade, experiments bear that the photon correlation, entanglement, and photon statistics are all well preserved in the coherent frequency upconversion [16-18].

Efficient sources of indistinguishable single photons are a key resource for various applications in fields like quantum sensing, quantum metrology and quantum information processing. In this contribution we report on single photon generation based on III-V semiconductor quantum dots (QDs). To increase the emission efficiency of single photons, it is essential to tailor the radiative properties of the quantum dot emitters by engineering their photonic environment. We present optimized single photon emitters being based on both micropillar and photonics crystal cavities, for applications in a vertical platform and on-chip in-plane platform, respectively. Electrically driven single photon sources with self assembled semiconductor QDs embedded into GaAs/AlAs micropillar cavities emit on demand net rates of ~35 MHz single photons, thus being well exploitable in quantum key distribution systems. In order to establish also a spatially deterministic fabrication platform, position controlled quantum dots are integrated into p-i-n micropillar cavities and single photon emission of a coupled QD-micropillar diode system is observed. Efficient broadband coupling of single photons into photonic crystal waveguides provides the basis for all on-chip quantum information processing, and an according approach is reported.

Recently, a quantum secure direct communication (QSDC) protocol based on the mixture of Bell state particles and single photons[Acta Phys. Sin. 65 230301(2016)] was put forward. In this QSDC protocol, the single photons and the Bell states were both used as information carriers. To be specific, each Bell state as well as single photon was encoded by three bits of classical information. After the sender told the receiver how to measure the particles, the receiver could read out the secret message sent by the sender. Speciously, the information transmission efficiency of this protocol was high. Unfortunately, there exists the information leakage problem in this protocol. When the sender announces that the receiver uses the Z-basis to measure a single photon, everyone knows that the sent secret message is 000 or 001, that is, the first two bits are leaked out; when the sender announces that the receiver uses the X-basis to measure a single photon, everyone knows that the sent secret message is 010 or 011, that is, the first two bits are leaked out too; when the sender announces that the receiver uses the Bell-basis to measure a pair of particles from a Bell state, everyone knows that the sent secret message is 100, 101, 110 or 111, that is, the first bit is leaked out. In a word, two of the three bits of classical information encoded in a single photon, and one of the three bits of classical information encoded in a Bell state are leaked out. Therefore, this scheme is not secure. On the basis of keeping the original idea and changing the contents of the protocol as less as possible, we put forward an improved message encoding rule to solve the information leakage problem, that is, the single photon is only encoded by one bit of classical information, and the Bell state is only encoded by two bits of classical information. In fact, this makes the information capacity of the improved protocol achieves the Helovo bound. So it has high coding capacity. We hope researchers pay more attention to the information leakage problem in quantum secure communication protocols, and thus design truly secure ones.

As currently implemented, single-photon sources cannot be made to produce single photons with high probability, while simultaneously suppressing the probability of yielding two or more photons. Because of this, single photon sources cannot really produce single photons on demand. We describe a multiplexed system that allows the probabilities of producing one and more photons to be adjusted independently, enabling a much better approximation of a source of single photons on demand. The scheme uses a heralded photon source based on parametric downconversion, but by effectively breaking the trigger detector area into multiple regions, we are able to extract more information about a heralded photon than is possible with a conventional arrangement. This scheme allows photons to be produced along with a quantitative “certification ” that they are single photons. Some of the single-photon certifications can be significantly better than what is possible with conventional downconversion sources (using a unified trigger detector region), as well as being better than faint laser sources. With such a source of more tightly certified single photons, it should be possible to improve the maximum secure bit rate possible over a quantum cryptographic link. We present an analysis of the relative merits of this method over the conventional arrangement.

The parametric interaction of light beams in nonlinear materials is usually thought to be too weak to be observed when the fields involved are at the single-photon level. However, such single-photon level nonlinearity is not only fundamentally fascinating but holds great potential for emerging technologies and applications involving heralding entanglement at a distance. Here we use a high-efficiency waveguide to demonstrate the sum-frequency generation between a single photon and a single-photon level coherent state. The use of an integrated, solid state, room temperature device and telecom wavelengths makes this type of system directly applicable to future quantum communication technologies such as device-independent quantum key distribution.

The Clean Air Mercury Rule (CAMR) which was published in the Federal Register on May 18, 2005, requires that calibration of mercury continuous emissions monitors (CEMs) be performed with NIST-traceable standards. Western Research Institute (WRI) is working closely with the Electric Power Research Institute (EPRI), the National Institute of Standards and Technology (NIST), and the Environmental Protection Agency (EPA) to facilitate the development of the experimental criteria for a NIST traceability protocol for dynamic elemental mercury vapor generators. The traceability protocol will be written by EPA. Traceability will be based on the actual analysis of the output of each calibration unit at several concentration levels ranging from about 2-40 ug/m{sup 3}, and this analysis will be directly traceable to analyses by NIST using isotope dilution inductively coupled plasma/mass spectrometry (ID ICP/MS) through a chain of analyses linking the calibration unit in the power plant to the NIST ID ICP/MS. Prior to this project, NIST did not provide a recommended mercury vapor pressure equation or list mercury vapor pressure in its vapor pressure database. The NIST Physical and Chemical Properties Division in Boulder, Colorado was subcontracted under this project to study the issue in detail and to recommend a mercury vapormore » pressure equation that the vendors of mercury vapor pressure calibration units can use to calculate the elemental mercury vapor concentration in an equilibrium chamber at a particular temperature. As part of this study, a preliminary evaluation of calibration units from five vendors was made. The work was performed by NIST in Gaithersburg, MD and Joe Rovani from WRI who traveled to NIST as a Visiting Scientist.« less

A Look at its Past Decade and a Gaze towards its Future. As the National Metrology Institute (NMI) for the United States, the National Institute of Standards and Technology (NIST), formerly the National Bureau of Standards, has provided measurement services, both calibrations and reference materials, for more than 100 years. Through these services, our customers have benefitted from our measurement capabilities and expertise in many areas, including amount of substance; dimensional metrology; electricity and magnetism; ionizing radiation; mass and related quantities; photometry and radiometry; thermodynamics; and time and frequency. NIST’s customers have also had access to some of the lowest measurement uncertainties available and a dependable way to establish traceability to the International System of Units (SI) [http://www.nist.gov/pml/wmd/metric/si-units.cfm].In response to the signing of the International Committee for Weights and Measures (CIPM) Mutual Recognition Arrangement (MRA), NIST first established an institution-wide quality system for the measurement services 10 years ago [http://www.bipm.org/en/cipm-mra/objectives.html]. NIST’s Quality System for Measurement Services has advanced the quality of service and measurements we provide our customers by fostering an environment in which NIST management and staff work towards continual improvement in the development and delivery of NIST measurement services. This paper describes NIST’s Quality System for the Measurement Services and its relevance to international standards of quality, such as the International Organization for Standardization and the International Electrotechnical Commission (ISO/IEC) 17025 standard and ISO Guide 34 [http://www.nist.gov/nistqs/]. It also provides a history of this quality system and a glimpse of future goals for improving its implementation.

Standards provide critical benefits across a wide variety of contexts, including safety and health, environmental protection, and quality of products and services. However, while these benefits are generally acknowledged, estimating the social and economic value of standards and determining how specific entities and activities influence their development require careful analysis. In October of 2018, the National Institute of Standards and Technology (NIST) asked the RAND Corporation to estimate the benefit of NIST’s research contributing to particular fire safety standards. The original objectives of the project were to (1) document the role of the NIST in the standards development process, (2) estimate the value these standards provide to society, and (3) thereby inform the economic value of NIST’s contribution to these standards. This report presents results for the first two objectives. Given that NIST’s contribution is one of several inputs combining to create these standards, NIST’s share of the credit for their value could not be quantified. Our analysis focused on case studies in standards for home smoke alarms and for protecting structures at the wildland-urban interface (WUI). Our analysis draws on a wide variety of qualitative and quantitative methods to holistically describe the impacts of these standards and NIST’s role in their development. The intended audience of this report includes those who work on fire safety research, fire safety standards, building codes, and technology transfer. The conclusions presented here may also be of interest for broader resource allocation and federal budget justification purposes. Finally, this report was written to be accessible to any interested members of the general public.

Single photon avalanche diodes (SPADs) are a key underpinning technology to many existing and emerging applications, including LIDAR for 3D imaging as well as quantum imaging, quantum encryption and quantum information applications. There is a growing demand for low-cost LIDAR systems for autonomous vehicles, particularly in the short-wave infrared (SWIR) spectral range, which enables long-range measurements whilst complying with eye-safety regulations and offers enhanced transmission through atmospheric obscurants like smoke and haze compared to systems operating in the near-infrared. Furthermore, for quantum-key distribution, single photons must be measured at telecoms wavelengths for compatibility with optical fibre networks. Ge-on-Si SPADs offer significant potential for low-cost SWIR single photon detection, with the ability to meet the price points required for these large emerging markets thanks to Si foundry compatibility. This contrasts with state-of-the-art SWIR SPADs based on InGaAs/InP, which are not only expensive but suffer from the effects of afterpulsing.Here, we present an overview of our work on the design, fabrication and characterisation of pseudo-planar Ge-on-Si detectors, with both operation in the Geiger mode (i.e. SPADs), as well as linear mode for avalanche photodiodes (APDs). The pseudo-planar SPAD design resulted in a step-change in performance compared to mesa-based SPADs, leading to high single-photon detection efficiencies (SPDEs) of 38 % at 1310 nm wavelength, and ultimately low noise equivalent powers of 7.7x10-17 W/Hz0.5 in 26 µm diameter pixels at 125 K, with single photon detection demonstrated up to 165 K. This was achieved by local ion-implantation of a charge-sheet layer, used to mediate the electric field between the Si avalanche layer and the Ge absorber, which in conjunction with a local p+Ge etched contact layer enabled a reduced E-field at etched sidewalls. These devices demonstrated over 100 X improvement in NEP compared to the most comparable Ge-on-Si mesa devices, and showed reduced afterpulsing compared to commercial InGaAs/InP devices when run in nominally identical operating conditions.In order to further optimise the technology, and gain insight into the device dynamics, we have simulated SPADs using TCAD process and device simulators, and developed custom-code to solve triggering probabilities using McIntyre’s model to understand the sensitivities of the detectors to the device design. Simulations are compared to experimental DCR measurements to probe sensitivities to surface passivation and geometry scaling and reveal that surfaces do not appear to be the limiting factor on performance, therefore validating the pseudo-planar architecture. Furthermore, with these simulation techniques, we have investigated potential enhancements achievable by the inclusion of an etched photonic crystal nano-hole array, which is known to enhance absorption and will therefore enhance SPDE. Here, we demonstrate the design trade-offs between enhanced SPDE performance, and the degradation of DCR that can be induced by etching surfaces into the device active area.Finally, we present recent results on surface normal Ge-on-Si APDs using the pseudo-planar architecture in devices with 2 µm thick Ge absorbers. Here, the benefits of the device architecture are demonstrated to be applicable to high performance in the linear mode. Devices are measured at room-temperature, and demonstrate ~0.40 A/W responsivity at unity gain at 1550 nm wavelength, with a maximum avalanche gain of ~100, and excess noise of 3.1 at a gain of 20; to our knowledge a record for any Ge-on-Si APD.

Narrow-band time-frequency entangled biphotons are generated from spontaneous four-wave mixing in cold atom clouds. The coherence time of the entangled biphotons can be extended to sub-microseconds by the slow light effect. The temporal wavefunction of the biphotons can be manipulated through modulating the spectral or spatial mode of the controlling laser beams. Concerning a pair of entangled biphoton and the resulting heralded single photon, it was commonly believed that, time-frequency entanglement damages the temporal purity of the single photon. However, the case is totally different for biphotons with long coherence time which is far beyond the time resolution of single-photondetectors. We demonstrate that, the single photon heralded from these time-frequency entangled biphotons is in a pure temporal state. Therefore, single photons are able to be shaped through the time-frequency entanglement with their partner photons, while the single photons could be found to be still in a pure state and thus useful for quantum information processing and communication technology.

Single photons are the key ingredient for many photonic quantum technologies including quantum key distribution and measurement-based quantum computing. However, it remains difficult to create devices with the appropriate specifications for use in non-laboratory environments. The optical microcavity platform provides an attractive route towards a room temperature single photon source device. Our ultra-small focused ion beam (FIB) milled open-access cavities offer enhancement of the spontaneous emission rate, tunability of the emission spectrum and increased light collection. The embedment of solid-state emitters within these cavities enables us to create a robust room temperature single photon source device, with the potential for high efficiencies and single photon purities. Defects such as the nitrogen-vacancy (NV) centre in diamond have been shown to be stable room-temperature sources of single photons. There are new single emitters emerging in two-dimensional materials such as hexagonal boron nitride (hBN). Here we present developments in room-temperature coupling of single defects to open-access microcavities of a planar-hemispherical geometry with mode volumes down to λ3. We report enhancements in the spectral density of photons into a single cavity mode, combined with improved single photon purities. It will be shown that the NV-cavity system provides a ~3% single photon emission efficiency with purities of up to 94%. The hBN-cavity system provides count rates >1Mcts/s into a single cavity mode with purities up to 96%. With these high single photon purities, such devices would be robust against photon number splitting attacks making them attractive for applications in quantum cryptography.