Room-temperature single-photon sources using solid-state emitters and open-access microcavities (Conference Presentation)

Single photon sources are essential building blocks for fundamental quantum optics, and quantum information networks. Their widespread use is currently hindered by impractical features, such as the need for operation at cryogenic temperatures and emission wavelengths lying outside telecom windows. Taking advantage of telecom technology and point defects in GaN crystals, we present, for the first time, the development of a fully-fibered source of single photons operating at room temperature, emitting photons in the telecom O-band and fulfilling the standards of telecom photonics. We characterise an emitter producting single photons at the wavelength of 1292 nm, a spectral broadening compatible with CWDM channels of 13 nm, and a brightness of 25 kcps per mW of pump power. The source shows a signal-to-noise ratio of 16.5 and a purity g(2)(0) = (5.9 ± 0.5) × 10-2 at room temperature, showing high potential for being integrated transportable quantum cryptography devices.

We report progress in the development of tunable room temperature triggered single photon sources based on single nitrogen-vacancy (NV) centres in nanodiamond coupled to open access optical micro-cavities. The feeding of fluorescence from an NV centre into the cavity mode increases the spectral density of the emission and results in an output stream of triggered single photons with spectral line width of order 1 nm, tunable in the range 640 - 700 nm. We record single photon purities exceeding 96% and estimated device efficiencies up to 3%. We compare performance using plano-concave microcavities with radii of curvature from 25 μm to 4 μm and show that up to 17% of the total emission is fed into the TEM00 mode. Pulsed Hanbury-Brown Twiss (HBT) interferometry shows that an improvement in single photon purity is facilitated due to the increased spectral density.

The characterization of the single photon response of the Hamamatsu R7600 multi-anode photomultiplier tube (MaPMT) is presented, in view of a possible application in Ring Imaging Cherenkov (RICH) detectors and high rate single photon counting applications in general. For most of the measurements the main source of single photons was a commercial blue LED biased with a small current of a few nA. The spectra obtained with this source match those obtained with Cherenkov light from a PbF2 crystal illuminated with a 22Na gamma source, confirming that the test signals are single photons. Dark current and cross-talk were measured at the single photoelectron level. The single photon response of the PMT was also studied as a function of the bias ratio between dynodes. The sensitivity to magnetic field up to 30 G and the effectiveness of three magnetic shields with different geometries were evaluated. Gain loss due to aging was also studied up to 2000 hours of operation at high counting rate.

Heralded single-photon source (HSPS) with competitive single photon purity and indistinguishability has become an essential resource for photonic quantum information processing. Here, for the first time, we proposed a theoretical regime to enhance heralded single-photons generation by multiplexing the degree of the freedom of orbital angular momentum (OAM) of down-converted entangled photon pairs emitted from a nonlinear crystal. Experimentally, a proof-of-principle experiment has been performed through multiplexing three OAM modes. We achieve a 47$\%$ enhancement in single photon rate. A second-order autocorrelation function $g^{(2)}(0)<0.5$ ensures our multiplexed heralded single photons with good single photon purity. We further indicate that an OAM-multiplexed HSPS with high quality can be constructed by generating higher dimensional entangled state and sorting them with high efficiency in OAM space. Our avenue may approach a good HSPS with the deterministic property.

Using cavity-enhanced non-degenerate parametric down-conversion, we have built a frequency tunable source of heralded single photons with a narrow bandwidth of 8 MHz, making it compatible with atomic quantum memories. The photon state is 70% pure single photon as characterized by a tomographic measurement and reconstruction of the quantum state, revealing a clearly negative Wigner function. Furthermore, it has a spectral brightness of ~1,500 photons/s per MHz bandwidth, making it one of the brightest single photon sources available. We also investigate the correlation function of the down-converted fields using a combination of two very distinct detection methods; photon counting and homodyne measurement.

In atomic-scale or quantum physics, an electromagnetic field is composed of photons, optical packets so small that a typical laser pointer with 1mW of power emits billions of them each second. Being able to take away or add a single photon in a light field at will would be useful for accurate engineering of quantum states. Such pure single photons are ideal for carrying and manipulating information in emerging quantum technologies, but generating them still is very challenging. In quantum physics, subtraction or addition of a photon is not a deterministic process. Instead, the probability is proportional to the number of photons originally in the electromagnetic field. This is described by the equation â|n〉 = √ n|n − 1〉 and â†|n〉 = √ n+ 1|n + 1〉, where â and ↠are annihilation and creation operators, respectively, representing the action of subtracting and adding a photon in a field composed of n photons.1 Such single-photon operations were limited to pure theoretical discussions until 2004, when Grangier and coworkers found a simple way to subtract a photon2 from a field. Passing through a beam splitter of high transmittivity, some photons can be split from the initial field. A ‘click’ detected in the photodetector in the reflected channel means one photon has been subtracted from the field: see Figure 1(a). When the initial field is composed of a small number of photons, the effect is dramatic and may even completely change the characteristics of the field. For example, let us take an initial single-mode squeezed state generated by ‘degenerate’ parametric down-conversion, which is an optical nonlinear process that converts a pump photon into two twin photons with half the pump photon energy. (This state is well known for its quantum noise squeezed into one quadrature at the expense of expanded noise in the other quadrature.) In order to visualize the noise properties and characteristics of the squeezed state, a probability-like function, such Figure 1. Setups to subtract (a) and add (b) a single photon from/to a light field. ρin and ρout denote the density operators of the input and output fields; BS is a low-reflectivity beam splitter; PDC is a nonlinear crystal where parametric down-conversion takes place; â and ↠denote on/off photodetectors.

The integration of a single photon source based on a solid-state emitter with a photonic structure remains challenging and specifically when it comes to be compatible with optical fibres. It is important to do so for quantum technologies where single photon sources constitute building blocks for many technologies. In this work, we demonstrate the integration of a single photon source, made of a colloidal semiconductor nanocrystal, with a photonic structure made of a glass waveguide obtained by the ion-exchange technique, which is a fibre-compatible platform used in telecom photonics. Using surface functionalisation and a secondary waveguide of titanium dioxide, we manage to couple single photons from the nanoemitter to the optical waveguide. We observe the single photon character is preserved and demonstrates a 1.2 Purcell factor. A coupling efficiency over 25% is expected thanks to the titanium dioxide secondary waveguiding layer, compared to around 2% obtained for simply positioning the nanocrystal on top of the waveguide alone. The optical waveguide is then pigtailed to an optical fibre to demonstrate a first proof of principle of an integrated single photon source at room temperature with a fibre-compatible platform made of glass with a coupling efficiency increase of 2.8.

Narrow-band time-frequency entangled biphotons are generated from spontaneous four-wave mixing in cold atom clouds. The coherence time of the entangled biphotons can be extended to sub-microseconds by the slow light effect. The temporal wavefunction of the biphotons can be manipulated through modulating the spectral or spatial mode of the controlling laser beams. Concerning a pair of entangled biphoton and the resulting heralded single photon, it was commonly believed that, time-frequency entanglement damages the temporal purity of the single photon. However, the case is totally different for biphotons with long coherence time which is far beyond the time resolution of single-photondetectors. We demonstrate that, the single photon heralded from these time-frequency entangled biphotons is in a pure temporal state. Therefore, single photons are able to be shaped through the time-frequency entanglement with their partner photons, while the single photons could be found to be still in a pure state and thus useful for quantum information processing and communication technology.

We describe the simplest single–photon encoding schemes and introduce the concept of a quantum optical gate. These gates can be used to build up arbitrary entangled states of many initially separate single photons. Experimental realization of such a gate involves the development of nonlinear phase shift elements sensitice at the single quantum level. We report our experimental efforts using linear optical elements and non–classical sources where we are able to demonstrate interference and entanglement of initially separate single–photon pulses.

Quantum Key Distribution (QKD) is important for a variety of quantum technologies. Here we demonstrate a free-space room temperature, discreet-variable QKD system using a bright Single photon sources (SPS) in hexagonal Boron Nitride (hBN).

Efficient sources of indistinguishable single photons are a key resource for various applications in fields like quantum sensing, quantum metrology and quantum information processing. In this contribution we report on single photon generation based on III-V semiconductor quantum dots (QDs). To increase the emission efficiency of single photons, it is essential to tailor the radiative properties of the quantum dot emitters by engineering their photonic environment. We present optimized single photon emitters being based on both micropillar and photonics crystal cavities, for applications in a vertical platform and on-chip in-plane platform, respectively. Electrically driven single photon sources with self assembled semiconductor QDs embedded into GaAs/AlAs micropillar cavities emit on demand net rates of ~35 MHz single photons, thus being well exploitable in quantum key distribution systems. In order to establish also a spatially deterministic fabrication platform, position controlled quantum dots are integrated into p-i-n micropillar cavities and single photon emission of a coupled QD-micropillar diode system is observed. Efficient broadband coupling of single photons into photonic crystal waveguides provides the basis for all on-chip quantum information processing, and an according approach is reported.

Recently, a quantum secure direct communication (QSDC) protocol based on the mixture of Bell state particles and single photons[Acta Phys. Sin. 65 230301(2016)] was put forward. In this QSDC protocol, the single photons and the Bell states were both used as information carriers. To be specific, each Bell state as well as single photon was encoded by three bits of classical information. After the sender told the receiver how to measure the particles, the receiver could read out the secret message sent by the sender. Speciously, the information transmission efficiency of this protocol was high. Unfortunately, there exists the information leakage problem in this protocol. When the sender announces that the receiver uses the Z-basis to measure a single photon, everyone knows that the sent secret message is 000 or 001, that is, the first two bits are leaked out; when the sender announces that the receiver uses the X-basis to measure a single photon, everyone knows that the sent secret message is 010 or 011, that is, the first two bits are leaked out too; when the sender announces that the receiver uses the Bell-basis to measure a pair of particles from a Bell state, everyone knows that the sent secret message is 100, 101, 110 or 111, that is, the first bit is leaked out. In a word, two of the three bits of classical information encoded in a single photon, and one of the three bits of classical information encoded in a Bell state are leaked out. Therefore, this scheme is not secure. On the basis of keeping the original idea and changing the contents of the protocol as less as possible, we put forward an improved message encoding rule to solve the information leakage problem, that is, the single photon is only encoded by one bit of classical information, and the Bell state is only encoded by two bits of classical information. In fact, this makes the information capacity of the improved protocol achieves the Helovo bound. So it has high coding capacity. We hope researchers pay more attention to the information leakage problem in quantum secure communication protocols, and thus design truly secure ones.

As currently implemented, single-photon sources cannot be made to produce single photons with high probability, while simultaneously suppressing the probability of yielding two or more photons. Because of this, single photon sources cannot really produce single photons on demand. We describe a multiplexed system that allows the probabilities of producing one and more photons to be adjusted independently, enabling a much better approximation of a source of single photons on demand. The scheme uses a heralded photon source based on parametric downconversion, but by effectively breaking the trigger detector area into multiple regions, we are able to extract more information about a heralded photon than is possible with a conventional arrangement. This scheme allows photons to be produced along with a quantitative “certification ” that they are single photons. Some of the single-photon certifications can be significantly better than what is possible with conventional downconversion sources (using a unified trigger detector region), as well as being better than faint laser sources. With such a source of more tightly certified single photons, it should be possible to improve the maximum secure bit rate possible over a quantum cryptographic link. We present an analysis of the relative merits of this method over the conventional arrangement.

Single semiconductor quantum dots have been extensively used to demonstrate the deterministic emission of high purity single photons. The single photon emission performance of these nanostructures has become very well controlled, offering high levels of photon indistinguishability and brightness. Ultimately, quantum technologies will require the development of a set of devices to manipulate and control the state of the photons. Here we measure and simulate a novel all-optical route to switch the single photon stream emitted from the excitonic transition in a single semiconductor quantum dot. A dual non-resonant excitation pumping scheme is used to engineer a switching device operated with GHz speeds, high differential contrasts, ultra-low power consumption and high single photon purity. Our device scheme can be replicated in many different zero dimensional semiconductors, providing a novel route towards developing a platform-independent on-chip design for high speed and low power consumption quantum devices.

The prototype of a quantum random number generator is a single photon which impinges onto a beam splitter and is then detected by single photon detectors at one of the two output paths. Prior to detection, the photon is in a quantum mechanical superposition state of the two possible outcomes with –ideally– equal amplitudes until its position is determined by measurement. When the two output modes are observed by a single photon detector, the generated clicks can be interpreted as ones and zeros – and a raw random bit stream is obtained. Here we implement such a random bit generator based on single photons from a defect center in diamond. We investigate the single photon emission of the defect center by an anti-bunching measurement. This certifies the “quantumness” of the supplied photonic input state, while the random “decision” is still based on the vacuum fluctuations at the open port of the beam-splitter. Technical limitations, such as intensity fluctuations, mechanical drift, and bias are discussed. A number of ways to suppress such unwanted effects, and an a priori entropy estimation are presented. The single photon nature allows for a characterization of the non-classicality of the source, and allows to determine a background fraction. Due to the NV-center’s superior stability and optical properties, we can operate the generator under ambient conditions around the clock. We present a true 24/7 operation of the implemented random bit generator.